Localized versus delocalized excitations just above the 3d threshold in krypton clusters studied by Auger electron spectroscopy
Tchaplyguine, Maxim LU ; Kivimäki, A ; Peredkov, Sergey LU ; Ristinmaa Sörensen, Stacey LU ; Rosso, Aldana LU ; Öhrwall, Gunnar LU
; Schulz, J
; Lundwall, M
; Björneholm, Olle
LU
and Mårtensson, N.
, et al.
(2007)
In Journal of Chemical Physics
127(12).
- Abstract
- We present Auger spectroscopy studies of large krypton clusters excited by soft x-ray photons with energies on and just above the 3d(5/2) ionization threshold. The deexcitation spectra contain new features as compared to the spectra measured both below and far above threshold. Possible origins of these extra features, which stay at constant kinetic energies, are discussed: (1) normal Auger process with a postcollision interaction induced energy shift, (2) recapture of photoelectrons into high Rydberg orbitals after Auger decay, and (3) excitation into the conduction band (or "internal" ionization) followed by Auger decay. The first two schemes are ruled out, hence internal ionization remains the most probable explanation. (C) 2007 American... (More)
- We present Auger spectroscopy studies of large krypton clusters excited by soft x-ray photons with energies on and just above the 3d(5/2) ionization threshold. The deexcitation spectra contain new features as compared to the spectra measured both below and far above threshold. Possible origins of these extra features, which stay at constant kinetic energies, are discussed: (1) normal Auger process with a postcollision interaction induced energy shift, (2) recapture of photoelectrons into high Rydberg orbitals after Auger decay, and (3) excitation into the conduction band (or "internal" ionization) followed by Auger decay. The first two schemes are ruled out, hence internal ionization remains the most probable explanation. (C) 2007 American Institute of Physics. (Less)
Please use this url to cite or link to this publication:
https://lup.lub.lu.se/record/764136
- author
- Tchaplyguine, Maxim
LU
; Kivimäki, A
; Peredkov, Sergey
LU
; Ristinmaa Sörensen, Stacey
LU
; Rosso, Aldana
LU
; Öhrwall, Gunnar
LU
; Schulz, J
; Lundwall, M
; Björneholm, Olle
LU
and Mårtensson, N.
, et al. (More)
- Tchaplyguine, Maxim
LU
; Kivimäki, A
; Peredkov, Sergey
LU
; Ristinmaa Sörensen, Stacey
LU
; Rosso, Aldana
LU
; Öhrwall, Gunnar
LU
; Schulz, J
; Lundwall, M
; Björneholm, Olle
LU
; Mårtensson, N.
; Rander, T.
and Lindblad, Andreas
LU
(Less)
- organization
- publishing date
- 2007
- type
- Contribution to journal
- publication status
- published
- subject
- in
- Journal of Chemical Physics
- volume
- 127
- issue
- 12
- article number
- 124314
- publisher
- American Institute of Physics (AIP)
- external identifiers
-
- wos:000249787300026
- scopus:34848823198
- ISSN
- 0021-9606
- DOI
- 10.1063/1.2770460
- language
- English
- LU publication?
- yes
- id
- d0106ace-e0ff-40b1-ba3b-795d2e7eb7fa (old id 764136)
- date added to LUP
- 2016-04-01 12:29:12
- date last changed
- 2022-01-27 05:43:14
@article{d0106ace-e0ff-40b1-ba3b-795d2e7eb7fa,
abstract = {{We present Auger spectroscopy studies of large krypton clusters excited by soft x-ray photons with energies on and just above the 3d(5/2) ionization threshold. The deexcitation spectra contain new features as compared to the spectra measured both below and far above threshold. Possible origins of these extra features, which stay at constant kinetic energies, are discussed: (1) normal Auger process with a postcollision interaction induced energy shift, (2) recapture of photoelectrons into high Rydberg orbitals after Auger decay, and (3) excitation into the conduction band (or "internal" ionization) followed by Auger decay. The first two schemes are ruled out, hence internal ionization remains the most probable explanation. (C) 2007 American Institute of Physics.}},
author = {{Tchaplyguine, Maxim and Kivimäki, A and Peredkov, Sergey and Ristinmaa Sörensen, Stacey and Rosso, Aldana and Öhrwall, Gunnar and Schulz, J and Lundwall, M and Björneholm, Olle and Mårtensson, N. and Rander, T. and Lindblad, Andreas}},
issn = {{0021-9606}},
language = {{eng}},
number = {{12}},
publisher = {{American Institute of Physics (AIP)}},
series = {{Journal of Chemical Physics}},
title = {{Localized versus delocalized excitations just above the 3d threshold in krypton clusters studied by Auger electron spectroscopy}},
url = {{http://dx.doi.org/10.1063/1.2770460}},
doi = {{10.1063/1.2770460}},
volume = {{127}},
year = {{2007}},
}