Electron extraction from excited quantum dots with higher order coulomb scattering

Kalaee, Alex Arash Sand; Wacker, Andreas (2020-03-19). Electron extraction from excited quantum dots with higher order coulomb scattering. Journal of Physics Communications, 4, (3)
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DOI:
| Published | English
Authors:
Kalaee, Alex Arash Sand ; Wacker, Andreas
Department:
Mathematical Physics
NanoLund: Centre for Nanoscience
Abstract:

The electron kinetics in nanowire-based hot-carrier solar cells is studied, where both relaxation and extraction are considered concurrently. Our kinetics is formulated in the many-particle basis of the interacting system. Detailed comparison with simplified calculations based on product states shows that this includes the Coulomb interaction both in lowest and higher orders. While relaxation rates of 1 ps are obtained, if lowest order processes are available, timescales of tens of ps arise if these are not allowed for particular designs and initial conditions. Based on these calculations we quantify the second order effects and discuss the extraction efficiency, which remains low unless an energy filter by resonant tunnelling is applied.

Keywords:
Hot-carrier solar cells ; Quantum kinetics ; Thermalisation
ISSN:
2399-6528
LUP-ID:
2b96d5d4-9f82-4900-859b-4aebb3d58d13 | Link: https://lup.lub.lu.se/record/2b96d5d4-9f82-4900-859b-4aebb3d58d13 | Statistics

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