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Frustrated tunneling dynamics in ultrashort laser pulses

Olofsson, Edvin LU ; Carlström, Stefanos LU and Dahlström, Jan Marcus LU (2021) In Journal of Physics B: Atomic, Molecular and Optical Physics 54(15).
Abstract

We study a model for frustrated tunneling ionization using ultrashort laser pulses. The model is based on the strong field approximation and it employs the saddle point approximation to predict quasiclassical trajectories that are captured on Rydberg states. We present a classification of the saddle-point solutions and explore their behavior as functions of angular momentum of the final state, as well as the carrier-envelope phase (CEP) of the laser pulse. We compare the final state population computed by the model to results obtained by numerical propagation of the time-dependent Schrödinger equation (TDSE) for the hydrogen atom. While we find qualitative agreement in the CEP dependence of the populations in principal quantum numbers,... (More)

We study a model for frustrated tunneling ionization using ultrashort laser pulses. The model is based on the strong field approximation and it employs the saddle point approximation to predict quasiclassical trajectories that are captured on Rydberg states. We present a classification of the saddle-point solutions and explore their behavior as functions of angular momentum of the final state, as well as the carrier-envelope phase (CEP) of the laser pulse. We compare the final state population computed by the model to results obtained by numerical propagation of the time-dependent Schrödinger equation (TDSE) for the hydrogen atom. While we find qualitative agreement in the CEP dependence of the populations in principal quantum numbers, n, the populations to individual angular momentum channels, ℓ, are found to be inconsistent between model and TDSE. Thus, our results show that improvements of the quasiclassical trajectories are in order for a quantitative model of frustrated tunneling ionization.

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author
; and
organization
publishing date
type
Contribution to journal
publication status
published
subject
keywords
frustrated tunneling, frustrated tunneling ionization, Keldysh theory, Rydberg atoms, strong-field approximation, strong-field ionization
in
Journal of Physics B: Atomic, Molecular and Optical Physics
volume
54
issue
15
article number
154002
publisher
IOP Publishing
external identifiers
  • scopus:85114812921
ISSN
0953-4075
DOI
10.1088/1361-6455/ac1ae4
language
English
LU publication?
yes
id
03b0c22e-c449-4c4e-912d-9cf31798d9f8
date added to LUP
2021-10-11 11:38:17
date last changed
2024-05-04 13:55:59
@article{03b0c22e-c449-4c4e-912d-9cf31798d9f8,
  abstract     = {{<p>We study a model for frustrated tunneling ionization using ultrashort laser pulses. The model is based on the strong field approximation and it employs the saddle point approximation to predict quasiclassical trajectories that are captured on Rydberg states. We present a classification of the saddle-point solutions and explore their behavior as functions of angular momentum of the final state, as well as the carrier-envelope phase (CEP) of the laser pulse. We compare the final state population computed by the model to results obtained by numerical propagation of the time-dependent Schrödinger equation (TDSE) for the hydrogen atom. While we find qualitative agreement in the CEP dependence of the populations in principal quantum numbers, n, the populations to individual angular momentum channels, ℓ, are found to be inconsistent between model and TDSE. Thus, our results show that improvements of the quasiclassical trajectories are in order for a quantitative model of frustrated tunneling ionization.</p>}},
  author       = {{Olofsson, Edvin and Carlström, Stefanos and Dahlström, Jan Marcus}},
  issn         = {{0953-4075}},
  keywords     = {{frustrated tunneling; frustrated tunneling ionization; Keldysh theory; Rydberg atoms; strong-field approximation; strong-field ionization}},
  language     = {{eng}},
  number       = {{15}},
  publisher    = {{IOP Publishing}},
  series       = {{Journal of Physics B: Atomic, Molecular and Optical Physics}},
  title        = {{Frustrated tunneling dynamics in ultrashort laser pulses}},
  url          = {{http://dx.doi.org/10.1088/1361-6455/ac1ae4}},
  doi          = {{10.1088/1361-6455/ac1ae4}},
  volume       = {{54}},
  year         = {{2021}},
}