Skip to main content

Lund University Publications

LUND UNIVERSITY LIBRARIES

Coherent soft X-ray pulses from an echo-enabled harmonic generation free-electron laser

Rebernik Ribič, P. ; Pop, Mihai LU and Allaria, E.M. (2019) In Nature Photonics 13. p.555-561
Abstract
X-ray free-electron lasers (FELs), which amplify light emitted by a relativistic electron beam, are extending nonlinear optical techniques to shorter wavelengths, adding element specificity by exciting and probing electronic transitions from core levels. These techniques would benefit tremendously from having a stable FEL source, generating spectrally pure and wavelength-tunable pulses. We show that such requirements can be met by operating the FEL in the so-called echo-enabled harmonic generation (EEHG) configuration. Here, two external conventional lasers are used to precisely tailor the longitudinal phase space of the electron beam before emission of X-rays. We demonstrate high-gain EEHG lasing producing stable, intense, nearly fully... (More)
X-ray free-electron lasers (FELs), which amplify light emitted by a relativistic electron beam, are extending nonlinear optical techniques to shorter wavelengths, adding element specificity by exciting and probing electronic transitions from core levels. These techniques would benefit tremendously from having a stable FEL source, generating spectrally pure and wavelength-tunable pulses. We show that such requirements can be met by operating the FEL in the so-called echo-enabled harmonic generation (EEHG) configuration. Here, two external conventional lasers are used to precisely tailor the longitudinal phase space of the electron beam before emission of X-rays. We demonstrate high-gain EEHG lasing producing stable, intense, nearly fully coherent pulses at wavelengths as short as 5.9 nm (~211 eV) at the FERMI FEL user facility. Low sensitivity to electron-beam imperfections and observation of stable, narrow-band, coherent emission down to 2.6 nm (~474 eV) make the technique a prime candidate for generating laser-like pulses in the X-ray spectral region, opening the door to multidimensional coherent spectroscopies at short wavelengths. © 2019, The Author(s), under exclusive licence to Springer Nature Limited. (Less)
Please use this url to cite or link to this publication:
author
; and
author collaboration
organization
publishing date
type
Contribution to journal
publication status
published
subject
keywords
Electron beams, Electron emission, Free electron lasers, Harmonic generation, Phase space methods, X rays, Coherent spectroscopies, Conventional lasers, Electronic transition, Element specificity, Harmonic generation free electron lasers, Nonlinear optical technique, Relativistic electron beam, X-ray free electron lasers, Electrons
in
Nature Photonics
volume
13
pages
555 - 561
publisher
Nature Publishing Group
external identifiers
  • scopus:85065323288
ISSN
1749-4885
DOI
10.1038/s41566-019-0427-1
language
English
LU publication?
yes
additional info
Export Date: 24 July 2019
id
0639be98-7c19-4bd7-b736-64d652dddf9e
date added to LUP
2019-07-24 14:37:18
date last changed
2022-04-26 03:15:36
@article{0639be98-7c19-4bd7-b736-64d652dddf9e,
  abstract     = {{X-ray free-electron lasers (FELs), which amplify light emitted by a relativistic electron beam, are extending nonlinear optical techniques to shorter wavelengths, adding element specificity by exciting and probing electronic transitions from core levels. These techniques would benefit tremendously from having a stable FEL source, generating spectrally pure and wavelength-tunable pulses. We show that such requirements can be met by operating the FEL in the so-called echo-enabled harmonic generation (EEHG) configuration. Here, two external conventional lasers are used to precisely tailor the longitudinal phase space of the electron beam before emission of X-rays. We demonstrate high-gain EEHG lasing producing stable, intense, nearly fully coherent pulses at wavelengths as short as 5.9 nm (~211 eV) at the FERMI FEL user facility. Low sensitivity to electron-beam imperfections and observation of stable, narrow-band, coherent emission down to 2.6 nm (~474 eV) make the technique a prime candidate for generating laser-like pulses in the X-ray spectral region, opening the door to multidimensional coherent spectroscopies at short wavelengths. © 2019, The Author(s), under exclusive licence to Springer Nature Limited.}},
  author       = {{Rebernik Ribič, P. and Pop, Mihai and Allaria, E.M.}},
  issn         = {{1749-4885}},
  keywords     = {{Electron beams; Electron emission; Free electron lasers; Harmonic generation; Phase space methods; X rays; Coherent spectroscopies; Conventional lasers; Electronic transition; Element specificity; Harmonic generation free electron lasers; Nonlinear optical technique; Relativistic electron beam; X-ray free electron lasers; Electrons}},
  language     = {{eng}},
  pages        = {{555--561}},
  publisher    = {{Nature Publishing Group}},
  series       = {{Nature Photonics}},
  title        = {{Coherent soft X-ray pulses from an echo-enabled harmonic generation free-electron laser}},
  url          = {{http://dx.doi.org/10.1038/s41566-019-0427-1}},
  doi          = {{10.1038/s41566-019-0427-1}},
  volume       = {{13}},
  year         = {{2019}},
}