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Molecular Movies from Molecular Frame Photoelectron Angular Distribution (MF-PAD) Measurements

Rouzée, Arnaud ; Huismans, Ymkje ; Kelkensberg, Freek ; Smolkowska, Aneta ; Jungmann, Julia H. ; Gijsbertsen, Arjan ; Siu, Wing Kiu ; Gademann, Georg ; Hundertmark, Axel and Johnsson, Per LU orcid , et al. (2014) In Springer Series in Chemical Physics 107. p.1-24
Abstract

We discuss recent and on-going experiments, where molecular frame photoelectron angular distributions (MFPADs) of high kinetic energy photoelectrons are measured in order to determine the time evolution of molecular structures in the course of a photochemical event. These experiments include, on the one hand, measurements where single XUV/X-ray photons, obtained from a free electron laser (FEL) or by means of high-harmonic generation (HHG), are used to eject a high energy photoelectron, and, on the other hand, measurements where a large number of mid-infrared photons are absorbed in the course of strong-field ionization. In the former case, first results indicate a manifestation of the both the electronic orbital and the molecular... (More)

We discuss recent and on-going experiments, where molecular frame photoelectron angular distributions (MFPADs) of high kinetic energy photoelectrons are measured in order to determine the time evolution of molecular structures in the course of a photochemical event. These experiments include, on the one hand, measurements where single XUV/X-ray photons, obtained from a free electron laser (FEL) or by means of high-harmonic generation (HHG), are used to eject a high energy photoelectron, and, on the other hand, measurements where a large number of mid-infrared photons are absorbed in the course of strong-field ionization. In the former case, first results indicate a manifestation of the both the electronic orbital and the molecular structure in the angle-resolved photoelectron distributions, while in the latter case novel holographic structures are measured that suggest that both the molecular structure and ultrafast electronic rearrangement processes can be studied with a time-resolution that reaches down into the attosecond and few-femtosecond domain.

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publishing date
type
Chapter in Book/Report/Conference proceeding
publication status
published
subject
host publication
Ultrafast Phenomena in Molecular Sciences : Femtosecond Physics and Chemistry - Femtosecond Physics and Chemistry
series title
Springer Series in Chemical Physics
volume
107
pages
24 pages
external identifiers
  • scopus:84886734519
ISSN
0172-6218
ISBN
9783319020501
DOI
10.1007/978-3-319-02051-8_1
language
English
LU publication?
yes
id
10e39ec8-8e6b-4c17-b699-e101dde634c7
date added to LUP
2018-06-29 13:47:39
date last changed
2021-09-22 02:28:06
@inbook{10e39ec8-8e6b-4c17-b699-e101dde634c7,
  abstract     = {<p>We discuss recent and on-going experiments, where molecular frame photoelectron angular distributions (MFPADs) of high kinetic energy photoelectrons are measured in order to determine the time evolution of molecular structures in the course of a photochemical event. These experiments include, on the one hand, measurements where single XUV/X-ray photons, obtained from a free electron laser (FEL) or by means of high-harmonic generation (HHG), are used to eject a high energy photoelectron, and, on the other hand, measurements where a large number of mid-infrared photons are absorbed in the course of strong-field ionization. In the former case, first results indicate a manifestation of the both the electronic orbital and the molecular structure in the angle-resolved photoelectron distributions, while in the latter case novel holographic structures are measured that suggest that both the molecular structure and ultrafast electronic rearrangement processes can be studied with a time-resolution that reaches down into the attosecond and few-femtosecond domain.</p>},
  author       = {Rouzée, Arnaud and Huismans, Ymkje and Kelkensberg, Freek and Smolkowska, Aneta and Jungmann, Julia H. and Gijsbertsen, Arjan and Siu, Wing Kiu and Gademann, Georg and Hundertmark, Axel and Johnsson, Per and Vrakking, Marc J J},
  booktitle    = {Ultrafast Phenomena in Molecular Sciences : Femtosecond Physics and Chemistry},
  isbn         = {9783319020501},
  issn         = {0172-6218},
  language     = {eng},
  month        = {01},
  pages        = {1--24},
  series       = {Springer Series in Chemical Physics},
  title        = {Molecular Movies from Molecular Frame Photoelectron Angular Distribution (MF-PAD) Measurements},
  url          = {http://dx.doi.org/10.1007/978-3-319-02051-8_1},
  doi          = {10.1007/978-3-319-02051-8_1},
  volume       = {107},
  year         = {2014},
}