The crystal structure of peroxymyoglobin generated through cryoradiolytic reduction of myoglobin compound III during data collection
(2008) In Biochemical Journal 412. p.257-264- Abstract
- Myoglobin has the ability to react with hydrogen peroxide, generating high-valent complexes similar to peroxidases (compounds I and II), and in the presence of excess hydrogen peroxide a third intermediate, compound III, with an oxymyoglobin-type structure is generated from compound II. The compound III is, however, easily one-electron reduced to peroxymyoglobin by synchrotron radiation during crystallograpic data collection. We have generated and solved the 1.30 angstrom (1 angstrom= 0.1 nin) resolution crystal structure of the peroxymyoglobin intermediate, which is isoelectric to compound 0 and has a Fe-O distance of 1.8 angstrom and O-O bond of 1.3 angstrom in accordance with a Fe-II-O-O- (or Fe-III-O-O2-) structure. The generation of... (More)
- Myoglobin has the ability to react with hydrogen peroxide, generating high-valent complexes similar to peroxidases (compounds I and II), and in the presence of excess hydrogen peroxide a third intermediate, compound III, with an oxymyoglobin-type structure is generated from compound II. The compound III is, however, easily one-electron reduced to peroxymyoglobin by synchrotron radiation during crystallograpic data collection. We have generated and solved the 1.30 angstrom (1 angstrom= 0.1 nin) resolution crystal structure of the peroxymyoglobin intermediate, which is isoelectric to compound 0 and has a Fe-O distance of 1.8 angstrom and O-O bond of 1.3 angstrom in accordance with a Fe-II-O-O- (or Fe-III-O-O2-) structure. The generation of the peroxy intermediate through reduction of compound III by X-rays shows the importance of using single-crystal microspectrophotometry when doing crystallography on metal loproteins. After having collected crystallographic data on a peroxy-generated myoglobin crystal, we were able (by a short annealing) to break the O-O bond leading to formation of compound II. These results indicate that the cryoradiolytic-generated peroxymyoglobin is biologically relevant through its conversion into compound II upon heating. Additionally, we have observed that the Xe1 site is occupied by a water molecule, which might be the leaving group in the compound II to compound III reaction. (Less)
Please use this url to cite or link to this publication:
https://lup.lub.lu.se/record/1201507
- author
- Hersleth, Hans-Petter ; Hsiao, Ya-Wen LU ; Ryde, Ulf LU ; Gorbitz, Carl Henrik and Andersson, K. Kristoffer
- organization
- publishing date
- 2008
- type
- Contribution to journal
- publication status
- published
- subject
- keywords
- oxygen binding, myoglobin, iron, cryoradiolytic, haem, peroxide complex
- in
- Biochemical Journal
- volume
- 412
- pages
- 257 - 264
- publisher
- Portland Press
- external identifiers
-
- wos:000256491900007
- scopus:44449131445
- pmid:18215120
- ISSN
- 0264-6021
- DOI
- 10.1042/BJ20070921
- language
- English
- LU publication?
- yes
- additional info
- The information about affiliations in this record was updated in December 2015. The record was previously connected to the following departments: Theoretical Chemistry (S) (011001039)
- id
- 485a845e-5cc9-4c6d-a1c0-154a8dbf327c (old id 1201507)
- date added to LUP
- 2016-04-01 14:29:13
- date last changed
- 2023-02-07 02:35:29
@article{485a845e-5cc9-4c6d-a1c0-154a8dbf327c, abstract = {{Myoglobin has the ability to react with hydrogen peroxide, generating high-valent complexes similar to peroxidases (compounds I and II), and in the presence of excess hydrogen peroxide a third intermediate, compound III, with an oxymyoglobin-type structure is generated from compound II. The compound III is, however, easily one-electron reduced to peroxymyoglobin by synchrotron radiation during crystallograpic data collection. We have generated and solved the 1.30 angstrom (1 angstrom= 0.1 nin) resolution crystal structure of the peroxymyoglobin intermediate, which is isoelectric to compound 0 and has a Fe-O distance of 1.8 angstrom and O-O bond of 1.3 angstrom in accordance with a Fe-II-O-O- (or Fe-III-O-O2-) structure. The generation of the peroxy intermediate through reduction of compound III by X-rays shows the importance of using single-crystal microspectrophotometry when doing crystallography on metal loproteins. After having collected crystallographic data on a peroxy-generated myoglobin crystal, we were able (by a short annealing) to break the O-O bond leading to formation of compound II. These results indicate that the cryoradiolytic-generated peroxymyoglobin is biologically relevant through its conversion into compound II upon heating. Additionally, we have observed that the Xe1 site is occupied by a water molecule, which might be the leaving group in the compound II to compound III reaction.}}, author = {{Hersleth, Hans-Petter and Hsiao, Ya-Wen and Ryde, Ulf and Gorbitz, Carl Henrik and Andersson, K. Kristoffer}}, issn = {{0264-6021}}, keywords = {{oxygen binding; myoglobin; iron; cryoradiolytic; haem; peroxide complex}}, language = {{eng}}, pages = {{257--264}}, publisher = {{Portland Press}}, series = {{Biochemical Journal}}, title = {{The crystal structure of peroxymyoglobin generated through cryoradiolytic reduction of myoglobin compound III during data collection}}, url = {{https://lup.lub.lu.se/search/files/136746075/108_myo0.pdf}}, doi = {{10.1042/BJ20070921}}, volume = {{412}}, year = {{2008}}, }