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Nonperturbative modeling of fifth-order coherent multidimensional spectroscopy in light harvesting antennas

Brueggemann, Ben and Pullerits, Tönu LU (2011) In New Journal of Physics 13(2).
Abstract
Recent advances in coherent multidimensional spectroscopy have boosted interest in exciton coherences in light harvesting complexes. We present nonperturbative calculations of two-dimensional (2D) electronic spectroscopy from a fifth-order phase-matching direction. The calculations show clear patterns that correspond to the electronic structure of one- and two-exciton manifolds of a Fenna-Matthews-Olsson light harvesting complex. Such signals can provide new information about the coherent properties of antenna pigment protein complexes.
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author
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organization
publishing date
type
Contribution to journal
publication status
published
subject
in
New Journal of Physics
volume
13
issue
2
article number
025024
publisher
IOP Publishing
external identifiers
  • wos:000287857400001
  • scopus:79952257004
ISSN
1367-2630
DOI
10.1088/1367-2630/13/2/025024
language
English
LU publication?
yes
additional info
The information about affiliations in this record was updated in December 2015. The record was previously connected to the following departments: Chemical Physics (S) (011001060)
id
f98c4e8e-52fd-4a86-92cf-a8a47d18f211 (old id 1868948)
date added to LUP
2016-04-01 13:58:39
date last changed
2020-12-08 05:02:45
@article{f98c4e8e-52fd-4a86-92cf-a8a47d18f211,
  abstract     = {Recent advances in coherent multidimensional spectroscopy have boosted interest in exciton coherences in light harvesting complexes. We present nonperturbative calculations of two-dimensional (2D) electronic spectroscopy from a fifth-order phase-matching direction. The calculations show clear patterns that correspond to the electronic structure of one- and two-exciton manifolds of a Fenna-Matthews-Olsson light harvesting complex. Such signals can provide new information about the coherent properties of antenna pigment protein complexes.},
  author       = {Brueggemann, Ben and Pullerits, Tönu},
  issn         = {1367-2630},
  language     = {eng},
  number       = {2},
  publisher    = {IOP Publishing},
  series       = {New Journal of Physics},
  title        = {Nonperturbative modeling of fifth-order coherent multidimensional spectroscopy in light harvesting antennas},
  url          = {http://dx.doi.org/10.1088/1367-2630/13/2/025024},
  doi          = {10.1088/1367-2630/13/2/025024},
  volume       = {13},
  year         = {2011},
}