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Low frequency spectroscopy of liquid water using THz-time domain spectroscopy.

Rönne, Cecilie LU and Keiding, S (2002) In Journal of Molecular Liquids 101(1-3). p.199-218
Abstract
In this paper we present an investigation of the dielectric response of H2O(1) and D2O(1) as a function of temperature from a supercooled state to near the boiling point. The data are obtained using THz-time domain spectroscopy, and covers the frequency range from 0 1-2 THz corresponding to 3 to 66 cm(-1). Before presenting the experimental results, we give a short introduction to some of the properties of liquid water, in particular the inter- and intramolecular motions responsible for the low frequency spectra, and brief introduction to the THz-time domain technique and its application as reflection spectroscopy is given. We also address recent theoretical and experimental contributions to the ongoing discussion regarding the microscopic... (More)
In this paper we present an investigation of the dielectric response of H2O(1) and D2O(1) as a function of temperature from a supercooled state to near the boiling point. The data are obtained using THz-time domain spectroscopy, and covers the frequency range from 0 1-2 THz corresponding to 3 to 66 cm(-1). Before presenting the experimental results, we give a short introduction to some of the properties of liquid water, in particular the inter- and intramolecular motions responsible for the low frequency spectra, and brief introduction to the THz-time domain technique and its application as reflection spectroscopy is given. We also address recent theoretical and experimental contributions to the ongoing discussion regarding the microscopic interpretation of the low frequency modes of liquid water. (C) 2002 Elsevier Science B.V. All rights reserved. (Less)
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author
organization
publishing date
type
Contribution to journal
publication status
published
subject
in
Journal of Molecular Liquids
volume
101
issue
1-3
pages
199 - 218
publisher
Elsevier
external identifiers
  • wos:000178067200018
  • scopus:0036836452
ISSN
0167-7322
DOI
10.1016/S0167-7322(02)00093-4
language
English
LU publication?
yes
id
8a3c941c-0fab-4c77-8558-e48a97f7c255 (old id 328552)
date added to LUP
2007-11-12 12:20:23
date last changed
2017-10-01 04:42:20
@article{8a3c941c-0fab-4c77-8558-e48a97f7c255,
  abstract     = {In this paper we present an investigation of the dielectric response of H2O(1) and D2O(1) as a function of temperature from a supercooled state to near the boiling point. The data are obtained using THz-time domain spectroscopy, and covers the frequency range from 0 1-2 THz corresponding to 3 to 66 cm(-1). Before presenting the experimental results, we give a short introduction to some of the properties of liquid water, in particular the inter- and intramolecular motions responsible for the low frequency spectra, and brief introduction to the THz-time domain technique and its application as reflection spectroscopy is given. We also address recent theoretical and experimental contributions to the ongoing discussion regarding the microscopic interpretation of the low frequency modes of liquid water. (C) 2002 Elsevier Science B.V. All rights reserved.},
  author       = {Rönne, Cecilie and Keiding, S},
  issn         = {0167-7322},
  language     = {eng},
  number       = {1-3},
  pages        = {199--218},
  publisher    = {Elsevier},
  series       = {Journal of Molecular Liquids},
  title        = {Low frequency spectroscopy of liquid water using THz-time domain spectroscopy.},
  url          = {http://dx.doi.org/10.1016/S0167-7322(02)00093-4},
  volume       = {101},
  year         = {2002},
}