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Nonstoichiometric Low-Temperature Grown GaAs Nanowires

Díaz Álvarez, Adrian ; Xu, Tao ; Tütüncüoglu, Gözde ; Demonchaux, Thomas ; Nys, Jean-Philippe ; Berthe, Maxime ; Matteini, Federico ; Potts, Heidi A LU ; Troadec, David and Patriarche, Gilles , et al. (2015) In Nano Letters 15(10). p.5-6440
Abstract

The structural and electronic properties of nonstoichiometric low-temperature grown GaAs nanowire shells have been investigated with scanning tunneling microscopy and spectroscopy, pump-probe reflectivity, and cathodoluminescence measurements. The growth of nonstoichiometric GaAs shells is achieved through the formation of As antisite defects, and to a lower extent, after annealing, As precipitates. Because of the high density of atomic steps on the nanowire sidewalls, the Fermi level is pinned midgap, causing the ionization of the subsurface antisites and the formation of depleted regions around the As precipitates. Controlling their incorporation offers a way to obtain unique electronic and optical properties that depart from the ones... (More)

The structural and electronic properties of nonstoichiometric low-temperature grown GaAs nanowire shells have been investigated with scanning tunneling microscopy and spectroscopy, pump-probe reflectivity, and cathodoluminescence measurements. The growth of nonstoichiometric GaAs shells is achieved through the formation of As antisite defects, and to a lower extent, after annealing, As precipitates. Because of the high density of atomic steps on the nanowire sidewalls, the Fermi level is pinned midgap, causing the ionization of the subsurface antisites and the formation of depleted regions around the As precipitates. Controlling their incorporation offers a way to obtain unique electronic and optical properties that depart from the ones found in conventional GaAs nanowires.

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publishing date
type
Contribution to journal
publication status
published
in
Nano Letters
volume
15
issue
10
pages
6 pages
publisher
The American Chemical Society (ACS)
external identifiers
  • pmid:26339987
  • scopus:84944339788
ISSN
1530-6992
DOI
10.1021/acs.nanolett.5b01802
language
English
LU publication?
no
id
32a75674-01d6-4f52-bb3b-a19cb5d30bc1
date added to LUP
2019-05-15 09:53:53
date last changed
2024-01-01 04:44:21
@article{32a75674-01d6-4f52-bb3b-a19cb5d30bc1,
  abstract     = {{<p>The structural and electronic properties of nonstoichiometric low-temperature grown GaAs nanowire shells have been investigated with scanning tunneling microscopy and spectroscopy, pump-probe reflectivity, and cathodoluminescence measurements. The growth of nonstoichiometric GaAs shells is achieved through the formation of As antisite defects, and to a lower extent, after annealing, As precipitates. Because of the high density of atomic steps on the nanowire sidewalls, the Fermi level is pinned midgap, causing the ionization of the subsurface antisites and the formation of depleted regions around the As precipitates. Controlling their incorporation offers a way to obtain unique electronic and optical properties that depart from the ones found in conventional GaAs nanowires. </p>}},
  author       = {{Díaz Álvarez, Adrian and Xu, Tao and Tütüncüoglu, Gözde and Demonchaux, Thomas and Nys, Jean-Philippe and Berthe, Maxime and Matteini, Federico and Potts, Heidi A and Troadec, David and Patriarche, Gilles and Lampin, Jean-François and Coinon, Christophe and Fontcuberta i Morral, Anna and Dunin-Borkowski, Rafal E and Ebert, Philipp and Grandidier, Bruno}},
  issn         = {{1530-6992}},
  language     = {{eng}},
  month        = {{10}},
  number       = {{10}},
  pages        = {{5--6440}},
  publisher    = {{The American Chemical Society (ACS)}},
  series       = {{Nano Letters}},
  title        = {{Nonstoichiometric Low-Temperature Grown GaAs Nanowires}},
  url          = {{http://dx.doi.org/10.1021/acs.nanolett.5b01802}},
  doi          = {{10.1021/acs.nanolett.5b01802}},
  volume       = {{15}},
  year         = {{2015}},
}