Experimental and theoretical studies of lifetimes and transition probabilities for Au II
(2002) In Journal of Physics B: Atomic, Molecular and Optical Physics 35(3). p.483-490- Abstract
- We report lifetime measurements for three of the 5d(9)6p levels in An II and relativistic multiconfiguration Dirac-Fock (MCDF) calculations of lifetimes and transitions probabilities in this ion. The work was motivated by significant disagreements between previous experimental 5d(9)6p lifetimes, obtained by means of the beam-foil (BF) method and theoretical data based on Hartree-Fock calculations in which relativistic effects were included as perturbations. The new measurements, based on laser-induced fluorescence, support the BF data and are also in excellent agreement with the MCDF results. We confirm that, while computational methods which include perturbative relativistic corrections appear to be adequate for moderately heavy elements... (More)
- We report lifetime measurements for three of the 5d(9)6p levels in An II and relativistic multiconfiguration Dirac-Fock (MCDF) calculations of lifetimes and transitions probabilities in this ion. The work was motivated by significant disagreements between previous experimental 5d(9)6p lifetimes, obtained by means of the beam-foil (BF) method and theoretical data based on Hartree-Fock calculations in which relativistic effects were included as perturbations. The new measurements, based on laser-induced fluorescence, support the BF data and are also in excellent agreement with the MCDF results. We confirm that, while computational methods which include perturbative relativistic corrections appear to be adequate for moderately heavy elements such as Ag, fully relativistic calculations are essential for describing systems as heavy as Au. (Less)
Please use this url to cite or link to this publication:
https://lup.lub.lu.se/record/342286
- author
- Zhiguo, Zhang LU ; Brage, Tomas LU ; Curtis, LJ ; Lundberg, Hans LU and Martinson, Indrek LU
- organization
- publishing date
- 2002
- type
- Contribution to journal
- publication status
- published
- subject
- in
- Journal of Physics B: Atomic, Molecular and Optical Physics
- volume
- 35
- issue
- 3
- pages
- 483 - 490
- publisher
- IOP Publishing
- external identifiers
-
- wos:000174258700008
- scopus:0037075136
- ISSN
- 0953-4075
- DOI
- 10.1088/0953-4075/35/3/303
- language
- English
- LU publication?
- yes
- id
- 14a358b7-9142-472f-bb92-bacd466e4059 (old id 342286)
- date added to LUP
- 2016-04-01 15:17:30
- date last changed
- 2022-01-28 04:37:42
@article{14a358b7-9142-472f-bb92-bacd466e4059,
abstract = {{We report lifetime measurements for three of the 5d(9)6p levels in An II and relativistic multiconfiguration Dirac-Fock (MCDF) calculations of lifetimes and transitions probabilities in this ion. The work was motivated by significant disagreements between previous experimental 5d(9)6p lifetimes, obtained by means of the beam-foil (BF) method and theoretical data based on Hartree-Fock calculations in which relativistic effects were included as perturbations. The new measurements, based on laser-induced fluorescence, support the BF data and are also in excellent agreement with the MCDF results. We confirm that, while computational methods which include perturbative relativistic corrections appear to be adequate for moderately heavy elements such as Ag, fully relativistic calculations are essential for describing systems as heavy as Au.}},
author = {{Zhiguo, Zhang and Brage, Tomas and Curtis, LJ and Lundberg, Hans and Martinson, Indrek}},
issn = {{0953-4075}},
language = {{eng}},
number = {{3}},
pages = {{483--490}},
publisher = {{IOP Publishing}},
series = {{Journal of Physics B: Atomic, Molecular and Optical Physics}},
title = {{Experimental and theoretical studies of lifetimes and transition probabilities for Au II}},
url = {{https://lup.lub.lu.se/search/files/4360223/2371302.pdf}},
doi = {{10.1088/0953-4075/35/3/303}},
volume = {{35}},
year = {{2002}},
}