Comparison of the electronic structure of PPV and its derivative DIOXA-PPV
(2006) In Chemical Physics 327(2-3). p.474-484- Abstract
- Electronic structure of two conjugated polymers, PPV and its derivative DIOXA-PPV, are studied by quantum-chemistry methods. Good agreement between the calculations and available experimental data validates the applied methods and enables us to draw conclusions about properties of excitons and polarons in these polymers. In particular, simultaneous use of different correlation plots in atomic site representation and transition densities in real space representation reveals electronic structure and spatial localization of the elementary excitations. The properties of the DIOXA-PPV are discussed in context of possible applications in molecular electronics devices. (c) 2006 Elsevier B.V. All rights reserved.
Please use this url to cite or link to this publication:
https://lup.lub.lu.se/record/392797
- author
- Sun, Mengtao LU ; Kjellberg, Pär LU ; Beenken, Wichard LU and Pullerits, Tönu LU
- organization
- publishing date
- 2006
- type
- Contribution to journal
- publication status
- published
- subject
- keywords
- site representation, intramolecular charge and energy transfer, electron-hole coherence, real-space representation
- in
- Chemical Physics
- volume
- 327
- issue
- 2-3
- pages
- 474 - 484
- publisher
- Elsevier
- external identifiers
-
- wos:000240650900033
- scopus:33748112776
- ISSN
- 0301-0104
- DOI
- 10.1016/j.chemphys.2006.05.031
- language
- English
- LU publication?
- yes
- additional info
- The information about affiliations in this record was updated in December 2015. The record was previously connected to the following departments: Chemical Physics (S) (011001060)
- id
- 6c3c9a1e-45d6-4a8f-b159-19b3021bd529 (old id 392797)
- date added to LUP
- 2016-04-01 15:47:21
- date last changed
- 2022-03-30 03:03:09
@article{6c3c9a1e-45d6-4a8f-b159-19b3021bd529, abstract = {{Electronic structure of two conjugated polymers, PPV and its derivative DIOXA-PPV, are studied by quantum-chemistry methods. Good agreement between the calculations and available experimental data validates the applied methods and enables us to draw conclusions about properties of excitons and polarons in these polymers. In particular, simultaneous use of different correlation plots in atomic site representation and transition densities in real space representation reveals electronic structure and spatial localization of the elementary excitations. The properties of the DIOXA-PPV are discussed in context of possible applications in molecular electronics devices. (c) 2006 Elsevier B.V. All rights reserved.}}, author = {{Sun, Mengtao and Kjellberg, Pär and Beenken, Wichard and Pullerits, Tönu}}, issn = {{0301-0104}}, keywords = {{site representation; intramolecular charge and energy transfer; electron-hole coherence; real-space representation}}, language = {{eng}}, number = {{2-3}}, pages = {{474--484}}, publisher = {{Elsevier}}, series = {{Chemical Physics}}, title = {{Comparison of the electronic structure of PPV and its derivative DIOXA-PPV}}, url = {{http://dx.doi.org/10.1016/j.chemphys.2006.05.031}}, doi = {{10.1016/j.chemphys.2006.05.031}}, volume = {{327}}, year = {{2006}}, }