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Circularly polarized RABBITT applied to a Rabi-cycling atom

Liao, Yijie ; Olofsson, Edvin LU ; Dahlström, Jan Marcus LU ; Pi, Liang Wen ; Zhou, Yueming and Lu, Peixiang (2024) In Physical Review A 109(4).
Abstract

We utilize the reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) technique to study the phase of a Rabi-cycling atom using circularly polarized extreme ultraviolet and infrared fields, where the infrared field induces Rabi oscillations between the 2s and 2p states of lithium. Autler-Townes splittings are observed in sidebands of the photoelectron spectra and the relative phases of outgoing electron wave packets are retrieved from the azimuthal angle. In this RABBITT scheme, more ionization pathways beyond the usual two-photon pathways are required. Our results show that the polar-angle-integrated and polar-angle-resolved RABBITT phases have different behaviors when the extreme ultraviolet and... (More)

We utilize the reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) technique to study the phase of a Rabi-cycling atom using circularly polarized extreme ultraviolet and infrared fields, where the infrared field induces Rabi oscillations between the 2s and 2p states of lithium. Autler-Townes splittings are observed in sidebands of the photoelectron spectra and the relative phases of outgoing electron wave packets are retrieved from the azimuthal angle. In this RABBITT scheme, more ionization pathways beyond the usual two-photon pathways are required. Our results show that the polar-angle-integrated and polar-angle-resolved RABBITT phases have different behaviors when the extreme ultraviolet and infrared fields have co- and counter-rotating circular polarizations, which are traced back to the different ionization channels according to the selection rules in these two cases and their competition relying on the propensity rule in laser-assisted photoionization.

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author
; ; ; ; and
organization
publishing date
type
Contribution to journal
publication status
published
subject
in
Physical Review A
volume
109
issue
4
article number
043104
publisher
American Physical Society
external identifiers
  • scopus:85189338975
ISSN
2469-9926
DOI
10.1103/PhysRevA.109.043104
language
English
LU publication?
yes
id
416facdc-57d5-49a1-816d-c2e2e1b1fb2c
date added to LUP
2024-04-26 15:11:33
date last changed
2024-05-10 16:39:51
@article{416facdc-57d5-49a1-816d-c2e2e1b1fb2c,
  abstract     = {{<p>We utilize the reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) technique to study the phase of a Rabi-cycling atom using circularly polarized extreme ultraviolet and infrared fields, where the infrared field induces Rabi oscillations between the 2s and 2p states of lithium. Autler-Townes splittings are observed in sidebands of the photoelectron spectra and the relative phases of outgoing electron wave packets are retrieved from the azimuthal angle. In this RABBITT scheme, more ionization pathways beyond the usual two-photon pathways are required. Our results show that the polar-angle-integrated and polar-angle-resolved RABBITT phases have different behaviors when the extreme ultraviolet and infrared fields have co- and counter-rotating circular polarizations, which are traced back to the different ionization channels according to the selection rules in these two cases and their competition relying on the propensity rule in laser-assisted photoionization.</p>}},
  author       = {{Liao, Yijie and Olofsson, Edvin and Dahlström, Jan Marcus and Pi, Liang Wen and Zhou, Yueming and Lu, Peixiang}},
  issn         = {{2469-9926}},
  language     = {{eng}},
  number       = {{4}},
  publisher    = {{American Physical Society}},
  series       = {{Physical Review A}},
  title        = {{Circularly polarized RABBITT applied to a Rabi-cycling atom}},
  url          = {{http://dx.doi.org/10.1103/PhysRevA.109.043104}},
  doi          = {{10.1103/PhysRevA.109.043104}},
  volume       = {{109}},
  year         = {{2024}},
}