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Role of gallium diffusion in the formation of a magnetically dead layer at the Y3Fe5 O12/Gd3Ga5 O12 epitaxial interface

Suturin, S. M. ; Korovin, A. M. ; Bursian, V. E. ; Lutsev, L. V. ; Bourobina, V. ; Yakovlev, N. L. ; Montecchi, M. ; Pasquali, L. ; Ukleev, V. and Vorobiev, A. , et al. (2018) In Physical Review Materials 2(10).
Abstract

We have clarified the origin of a magnetically dead interface layer formed in yttrium iron garnet (YIG) films grown at above 700 °C onto a gadolinium gallium garnet (GGG) substrate by means of laser molecular beam epitaxy. The diffusion-assisted formation of a Ga-rich region at the YIG/GGG interface is demonstrated by means of composition depth profiling performed by x-ray photoelectron spectroscopy, secondary ion mass spectroscopy, and x-ray and neutron reflectometry. Our finding is in sharp contrast to the earlier expressed assumption that Gd acts as a migrant element in the YIG/GGG system. We further correlate the presence of a Ga-rich transition layer with considerable quenching of ferromagnetic resonance and spin wave propagation... (More)

We have clarified the origin of a magnetically dead interface layer formed in yttrium iron garnet (YIG) films grown at above 700 °C onto a gadolinium gallium garnet (GGG) substrate by means of laser molecular beam epitaxy. The diffusion-assisted formation of a Ga-rich region at the YIG/GGG interface is demonstrated by means of composition depth profiling performed by x-ray photoelectron spectroscopy, secondary ion mass spectroscopy, and x-ray and neutron reflectometry. Our finding is in sharp contrast to the earlier expressed assumption that Gd acts as a migrant element in the YIG/GGG system. We further correlate the presence of a Ga-rich transition layer with considerable quenching of ferromagnetic resonance and spin wave propagation in thin YIG films. Finally, we clarify the origin of the enigmatic low-density overlayer that is often observed in neutron and x-ray reflectometry studies of the YIG/GGG epitaxial system.

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publishing date
type
Contribution to journal
publication status
published
subject
in
Physical Review Materials
volume
2
issue
10
article number
104404
publisher
American Physical Society
external identifiers
  • scopus:85056267369
ISSN
2475-9953
DOI
10.1103/PhysRevMaterials.2.104404
language
English
LU publication?
no
id
42e33cf3-c922-4454-a3c2-91be32f0f4e3
date added to LUP
2022-04-04 13:08:35
date last changed
2022-04-04 17:01:02
@article{42e33cf3-c922-4454-a3c2-91be32f0f4e3,
  abstract     = {{<p>We have clarified the origin of a magnetically dead interface layer formed in yttrium iron garnet (YIG) films grown at above 700 °C onto a gadolinium gallium garnet (GGG) substrate by means of laser molecular beam epitaxy. The diffusion-assisted formation of a Ga-rich region at the YIG/GGG interface is demonstrated by means of composition depth profiling performed by x-ray photoelectron spectroscopy, secondary ion mass spectroscopy, and x-ray and neutron reflectometry. Our finding is in sharp contrast to the earlier expressed assumption that Gd acts as a migrant element in the YIG/GGG system. We further correlate the presence of a Ga-rich transition layer with considerable quenching of ferromagnetic resonance and spin wave propagation in thin YIG films. Finally, we clarify the origin of the enigmatic low-density overlayer that is often observed in neutron and x-ray reflectometry studies of the YIG/GGG epitaxial system.</p>}},
  author       = {{Suturin, S. M. and Korovin, A. M. and Bursian, V. E. and Lutsev, L. V. and Bourobina, V. and Yakovlev, N. L. and Montecchi, M. and Pasquali, L. and Ukleev, V. and Vorobiev, A. and Devishvili, A. and Sokolov, N. S.}},
  issn         = {{2475-9953}},
  language     = {{eng}},
  number       = {{10}},
  publisher    = {{American Physical Society}},
  series       = {{Physical Review Materials}},
  title        = {{Role of gallium diffusion in the formation of a magnetically dead layer at the Y3Fe5 O12/Gd3Ga5 O12 epitaxial interface}},
  url          = {{http://dx.doi.org/10.1103/PhysRevMaterials.2.104404}},
  doi          = {{10.1103/PhysRevMaterials.2.104404}},
  volume       = {{2}},
  year         = {{2018}},
}