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Rydberg-Resolved Resonant Inelastic Soft X-Ray Scattering: Dynamics at Core Ionization Thresholds

Rubensson, J. -E. ; Söderström, J. ; Binggeli, C. ; Gråsjö, J. ; Andersson, J. ; Såthe, Conny LU ; Hennies, Franz LU ; Bisogni, V. ; Huang, Y. and Olalde, P. , et al. (2015) In Physical Review Letters 114(13).
Abstract
Resonant inelastic x-ray scattering spectra excited in the immediate vicinity of the core-level ionization thresholds of N-2 have been recorded. Final states of well-resolved symmetry-selected Rydberg series converging to valence-level ionization thresholds with vibrational excitations are observed. The results are well described by a quasi-two-step model which assumes that the excited electron is unaffected by the radiative decay. This threshold dynamics simplifies the interpretation of resonant inelastic x-ray scattering spectra considerably and facilitates characterization of low-energy excited final states in molecular systems.
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organization
publishing date
type
Contribution to journal
publication status
published
subject
in
Physical Review Letters
volume
114
issue
13
article number
133001
publisher
American Physical Society
external identifiers
  • wos:000352073600001
  • pmid:25884123
  • pmid:25884123
  • scopus:85051953418
ISSN
1079-7114
DOI
10.1103/PhysRevLett.114.133001
language
English
LU publication?
yes
id
4eef5fcc-9a21-4df0-af7d-5688dcb80386 (old id 5277865)
date added to LUP
2016-04-01 09:52:32
date last changed
2022-04-04 00:09:36
@article{4eef5fcc-9a21-4df0-af7d-5688dcb80386,
  abstract     = {{Resonant inelastic x-ray scattering spectra excited in the immediate vicinity of the core-level ionization thresholds of N-2 have been recorded. Final states of well-resolved symmetry-selected Rydberg series converging to valence-level ionization thresholds with vibrational excitations are observed. The results are well described by a quasi-two-step model which assumes that the excited electron is unaffected by the radiative decay. This threshold dynamics simplifies the interpretation of resonant inelastic x-ray scattering spectra considerably and facilitates characterization of low-energy excited final states in molecular systems.}},
  author       = {{Rubensson, J. -E. and Söderström, J. and Binggeli, C. and Gråsjö, J. and Andersson, J. and Såthe, Conny and Hennies, Franz and Bisogni, V. and Huang, Y. and Olalde, P. and Schmitt, T. and Strocov, V. N. and Föhlisch, A. and Kennedy, B. and Pietzsch, A.}},
  issn         = {{1079-7114}},
  language     = {{eng}},
  number       = {{13}},
  publisher    = {{American Physical Society}},
  series       = {{Physical Review Letters}},
  title        = {{Rydberg-Resolved Resonant Inelastic Soft X-Ray Scattering: Dynamics at Core Ionization Thresholds}},
  url          = {{http://dx.doi.org/10.1103/PhysRevLett.114.133001}},
  doi          = {{10.1103/PhysRevLett.114.133001}},
  volume       = {{114}},
  year         = {{2015}},
}