Skip to main content

Lund University Publications

LUND UNIVERSITY LIBRARIES

Experimental evidence of monolayer arsenene : An exotic 2D semiconducting material

Shah, J. ; Wang, W. LU orcid ; Sohail, H. M. and Uhrberg, R. I.G. (2020) In 2D Materials 7(2).
Abstract

Group V element analogues of graphene have attracted a lot of attention recently due to their semiconducting band structures and several other interesting properties predicted by theoretical investigations in the literature. In this study, we present atomic and electronic structure data of an arsenic (As) layer on Ag(1 1 1). Low-energy electron diffraction and scanning tunneling microscopy data provide evidence for an ordered layer with a lattice constant of 3.6 Å. This value fits with the theoretical range of 3.54-3.64 Å for buckled arsenene, which is the structure consistently predicted by various theoretical studies. The electronic structure obtained by angle-resolved photoelectron spectroscopy shows the existence of three 2D... (More)

Group V element analogues of graphene have attracted a lot of attention recently due to their semiconducting band structures and several other interesting properties predicted by theoretical investigations in the literature. In this study, we present atomic and electronic structure data of an arsenic (As) layer on Ag(1 1 1). Low-energy electron diffraction and scanning tunneling microscopy data provide evidence for an ordered layer with a lattice constant of 3.6 Å. This value fits with the theoretical range of 3.54-3.64 Å for buckled arsenene, which is the structure consistently predicted by various theoretical studies. The electronic structure obtained by angle-resolved photoelectron spectroscopy shows the existence of three 2D electron bands within 4 eV below the Fermi level. The number of bands and the agreement between experimental band dispersions and the theoretical band structure provide further evidence for the formation of monolayer buckled arsenene on Ag(1 1 1).

(Less)
Please use this url to cite or link to this publication:
author
; ; and
organization
publishing date
type
Contribution to journal
publication status
published
subject
keywords
2D material, ARPES, arsenene, DFT, STM
in
2D Materials
volume
7
issue
2
article number
025013
publisher
IOP Publishing
external identifiers
  • scopus:85081662512
ISSN
2053-1583
DOI
10.1088/2053-1583/ab64fb
language
English
LU publication?
yes
id
6869f4c1-e776-41c1-8838-8a37d900b6c3
date added to LUP
2020-12-18 12:49:45
date last changed
2022-04-26 22:42:10
@article{6869f4c1-e776-41c1-8838-8a37d900b6c3,
  abstract     = {{<p>Group V element analogues of graphene have attracted a lot of attention recently due to their semiconducting band structures and several other interesting properties predicted by theoretical investigations in the literature. In this study, we present atomic and electronic structure data of an arsenic (As) layer on Ag(1 1 1). Low-energy electron diffraction and scanning tunneling microscopy data provide evidence for an ordered layer with a lattice constant of 3.6 Å. This value fits with the theoretical range of 3.54-3.64 Å for buckled arsenene, which is the structure consistently predicted by various theoretical studies. The electronic structure obtained by angle-resolved photoelectron spectroscopy shows the existence of three 2D electron bands within 4 eV below the Fermi level. The number of bands and the agreement between experimental band dispersions and the theoretical band structure provide further evidence for the formation of monolayer buckled arsenene on Ag(1 1 1).</p>}},
  author       = {{Shah, J. and Wang, W. and Sohail, H. M. and Uhrberg, R. I.G.}},
  issn         = {{2053-1583}},
  keywords     = {{2D material; ARPES; arsenene; DFT; STM}},
  language     = {{eng}},
  number       = {{2}},
  publisher    = {{IOP Publishing}},
  series       = {{2D Materials}},
  title        = {{Experimental evidence of monolayer arsenene : An exotic 2D semiconducting material}},
  url          = {{http://dx.doi.org/10.1088/2053-1583/ab64fb}},
  doi          = {{10.1088/2053-1583/ab64fb}},
  volume       = {{7}},
  year         = {{2020}},
}