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An external beam PIXE/PESA setup for characterization of fine aerosols

Martinsson, Bengt G. LU (1987) In Nuclear Inst. and Methods in Physics Research, B 22(1-3). p.356-363
Abstract

An external beam setup has been developed for the determination of elemental concentrations in fine aerosols (aerodynamic particle diameter less than about 2 μm). Carbon, nitrogen and oxygen are determined with particle elastic scattering analysis (PESA) and, simultaneously, elements heavier than silicon with PIXE at a proton energy of 3.58 MeV. Earlier work on aerosols with PESA and most PIXE work have been performed with the aerosol sample in high vacuum, which causes losses of certain compounds, e.g. several organic substances present in atmospheric aerosols. These losses are increased by the heating effect of the beam. The rate of mass loss of different aliphatic hydrocarbons has been investigated for different chamber gas... (More)

An external beam setup has been developed for the determination of elemental concentrations in fine aerosols (aerodynamic particle diameter less than about 2 μm). Carbon, nitrogen and oxygen are determined with particle elastic scattering analysis (PESA) and, simultaneously, elements heavier than silicon with PIXE at a proton energy of 3.58 MeV. Earlier work on aerosols with PESA and most PIXE work have been performed with the aerosol sample in high vacuum, which causes losses of certain compounds, e.g. several organic substances present in atmospheric aerosols. These losses are increased by the heating effect of the beam. The rate of mass loss of different aliphatic hydrocarbons has been investigated for different chamber gas pressures, chamber gas exchange rates and beam current densities. The external beam approach showed a considerable improvement compared with high vacuum analysis. The external beam setup is described in some detail with respect to geometry, electronics and the chamber gas-handling system.

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author
organization
publishing date
type
Contribution to journal
publication status
published
subject
in
Nuclear Inst. and Methods in Physics Research, B
volume
22
issue
1-3
pages
8 pages
publisher
Elsevier
external identifiers
  • scopus:0022685311
ISSN
0168-583X
DOI
10.1016/0168-583X(87)90358-2
language
English
LU publication?
yes
id
7d492838-cf02-4915-abb3-8460f7a20c12
date added to LUP
2019-05-16 09:51:57
date last changed
2021-01-03 10:02:14
@article{7d492838-cf02-4915-abb3-8460f7a20c12,
  abstract     = {{<p>An external beam setup has been developed for the determination of elemental concentrations in fine aerosols (aerodynamic particle diameter less than about 2 μm). Carbon, nitrogen and oxygen are determined with particle elastic scattering analysis (PESA) and, simultaneously, elements heavier than silicon with PIXE at a proton energy of 3.58 MeV. Earlier work on aerosols with PESA and most PIXE work have been performed with the aerosol sample in high vacuum, which causes losses of certain compounds, e.g. several organic substances present in atmospheric aerosols. These losses are increased by the heating effect of the beam. The rate of mass loss of different aliphatic hydrocarbons has been investigated for different chamber gas pressures, chamber gas exchange rates and beam current densities. The external beam approach showed a considerable improvement compared with high vacuum analysis. The external beam setup is described in some detail with respect to geometry, electronics and the chamber gas-handling system.</p>}},
  author       = {{Martinsson, Bengt G.}},
  issn         = {{0168-583X}},
  language     = {{eng}},
  month        = {{03}},
  number       = {{1-3}},
  pages        = {{356--363}},
  publisher    = {{Elsevier}},
  series       = {{Nuclear Inst. and Methods in Physics Research, B}},
  title        = {{An external beam PIXE/PESA setup for characterization of fine aerosols}},
  url          = {{http://dx.doi.org/10.1016/0168-583X(87)90358-2}},
  doi          = {{10.1016/0168-583X(87)90358-2}},
  volume       = {{22}},
  year         = {{1987}},
}