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Carriers, Quasi-particles, and Collective Excitations in Halide Perovskites

Fu, Jianhui ; Ramesh, Sankaran LU orcid ; Lim, Jia Wei Melvin and Sum, Tze Chien (2023) In Chemical Reviews
Abstract
Halide perovskites (HPs) are potential game-changing materials for a broad spectrum of optoelectronic applications ranging from photovoltaics, light-emitting devices, lasers to radiation detectors, ferroelectrics, thermoelectrics, etc. Underpinning this spectacular expansion is their fascinating photophysics involving a complex interplay of carrier, lattice, and quasi-particle interactions spanning several temporal orders that give rise to their remarkable optical and electronic properties. Herein, we critically examine and distill their dynamical behavior, collective interactions, and underlying mechanisms in conjunction with the experimental approaches. This review aims to provide a unified photophysical picture fundamental to... (More)
Halide perovskites (HPs) are potential game-changing materials for a broad spectrum of optoelectronic applications ranging from photovoltaics, light-emitting devices, lasers to radiation detectors, ferroelectrics, thermoelectrics, etc. Underpinning this spectacular expansion is their fascinating photophysics involving a complex interplay of carrier, lattice, and quasi-particle interactions spanning several temporal orders that give rise to their remarkable optical and electronic properties. Herein, we critically examine and distill their dynamical behavior, collective interactions, and underlying mechanisms in conjunction with the experimental approaches. This review aims to provide a unified photophysical picture fundamental to understanding the outstanding light-harvesting and light-emitting properties of HPs. The hotbed of carrier and quasi-particle interactions uncovered in HPs underscores the critical role of ultrafast spectroscopy and fundamental photophysics studies in advancing perovskite optoelectronics. (Less)
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author
; ; and
publishing date
type
Contribution to journal
publication status
published
subject
keywords
Excitons, Phonons, Perovskite, Quasi-particles, Spectroscopy
in
Chemical Reviews
publisher
The American Chemical Society (ACS)
external identifiers
  • scopus:85163967110
  • pmid:37276018
ISSN
1520-6890
DOI
10.1021/acs.chemrev.2c00843
language
English
LU publication?
no
id
822bfad2-fb29-4b4b-ab9e-0d23b0b4762b
date added to LUP
2023-06-22 21:37:45
date last changed
2023-09-22 03:00:12
@article{822bfad2-fb29-4b4b-ab9e-0d23b0b4762b,
  abstract     = {{Halide perovskites (HPs) are potential game-changing materials for a broad spectrum of optoelectronic applications ranging from photovoltaics, light-emitting devices, lasers to radiation detectors, ferroelectrics, thermoelectrics, etc. Underpinning this spectacular expansion is their fascinating photophysics involving a complex interplay of carrier, lattice, and quasi-particle interactions spanning several temporal orders that give rise to their remarkable optical and electronic properties. Herein, we critically examine and distill their dynamical behavior, collective interactions, and underlying mechanisms in conjunction with the experimental approaches. This review aims to provide a unified photophysical picture fundamental to understanding the outstanding light-harvesting and light-emitting properties of HPs. The hotbed of carrier and quasi-particle interactions uncovered in HPs underscores the critical role of ultrafast spectroscopy and fundamental photophysics studies in advancing perovskite optoelectronics.}},
  author       = {{Fu, Jianhui and Ramesh, Sankaran and Lim, Jia Wei Melvin and Sum, Tze Chien}},
  issn         = {{1520-6890}},
  keywords     = {{Excitons; Phonons; Perovskite; Quasi-particles; Spectroscopy}},
  language     = {{eng}},
  month        = {{07}},
  publisher    = {{The American Chemical Society (ACS)}},
  series       = {{Chemical Reviews}},
  title        = {{Carriers, Quasi-particles, and Collective Excitations in Halide Perovskites}},
  url          = {{http://dx.doi.org/10.1021/acs.chemrev.2c00843}},
  doi          = {{10.1021/acs.chemrev.2c00843}},
  year         = {{2023}},
}