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Spectroscopic techniques using synchrotron radiation and free-electron and conventional lasers

Tadjeddine, A.; Peremans, A.; Le Rille, A.; Zheng, W. Q.; Ortéga, J. M.; Glotin, F.; Prazeres, R.; Meyer, Michael; Lacoursière, J. and Nahon, L., et al. (1998) In Journal of Synchrotron Radiation 5(3). p.293-298
Abstract

Considerable progress in the investigation of the electronic and vibrational properties of atoms, molecules, materials, surfaces and interfaces has been achieved by combining different photon sources of complementary characteristics. In this paper some experimental results obtained recently at LURE by using two synchronized sources, such as the IR free-electron laser (FEL) CLIO, the VUV storage ring FEL, synchrotron radiation and table lasers, are presented. Using CLIO synchronized with a YAG laser allows the investigation of the vibrational properties of adsorbed species by the non-linear optical technique of visible-IR sum (difference) frequency generation, as shown for the adsorption of hydrogen on platinum in the electrochemical... (More)

Considerable progress in the investigation of the electronic and vibrational properties of atoms, molecules, materials, surfaces and interfaces has been achieved by combining different photon sources of complementary characteristics. In this paper some experimental results obtained recently at LURE by using two synchronized sources, such as the IR free-electron laser (FEL) CLIO, the VUV storage ring FEL, synchrotron radiation and table lasers, are presented. Using CLIO synchronized with a YAG laser allows the investigation of the vibrational properties of adsorbed species by the non-linear optical technique of visible-IR sum (difference) frequency generation, as shown for the adsorption of hydrogen on platinum in the electrochemical environment. The second result reported here relates to the study of the intersubband stimulated emission in GaAs/GaAlAs quantum wells by pump-probe experiments using the two-colour configuration of CLIO. The combination of a mode-locked Ar+ laser and synchrotron radiation has been used for investigations in a pump-probe arrangement of the ionization of Xe atoms via the resonant state Xe* 5p55d [3/2]1. The final example is a time-resolved core-level spectroscopy study of photoexcited Si(111) 2 × 1 surfaces by using a combination of the naturally synchronized UV storage ring laser and synchrotron radiation.

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publishing date
type
Contribution to journal
publication status
published
subject
keywords
Free-electron lasers, Spectroscopy, Two-colour configurations
in
Journal of Synchrotron Radiation
volume
5
issue
3
pages
6 pages
publisher
Wiley-Blackwell
external identifiers
  • scopus:0032382494
ISSN
0909-0495
DOI
10.1107/S0909049597015392
language
English
LU publication?
no
id
85b6ddc0-bdbb-4ebd-83ba-4de4e1f1d7a3
date added to LUP
2017-11-23 14:13:54
date last changed
2017-11-30 11:13:30
@article{85b6ddc0-bdbb-4ebd-83ba-4de4e1f1d7a3,
  abstract     = {<p>Considerable progress in the investigation of the electronic and vibrational properties of atoms, molecules, materials, surfaces and interfaces has been achieved by combining different photon sources of complementary characteristics. In this paper some experimental results obtained recently at LURE by using two synchronized sources, such as the IR free-electron laser (FEL) CLIO, the VUV storage ring FEL, synchrotron radiation and table lasers, are presented. Using CLIO synchronized with a YAG laser allows the investigation of the vibrational properties of adsorbed species by the non-linear optical technique of visible-IR sum (difference) frequency generation, as shown for the adsorption of hydrogen on platinum in the electrochemical environment. The second result reported here relates to the study of the intersubband stimulated emission in GaAs/GaAlAs quantum wells by pump-probe experiments using the two-colour configuration of CLIO. The combination of a mode-locked Ar<sup>+</sup> laser and synchrotron radiation has been used for investigations in a pump-probe arrangement of the ionization of Xe atoms via the resonant state Xe* 5p<sup>5</sup>5d [3/2]<sub>1</sub>. The final example is a time-resolved core-level spectroscopy study of photoexcited Si(111) 2 × 1 surfaces by using a combination of the naturally synchronized UV storage ring laser and synchrotron radiation.</p>},
  author       = {Tadjeddine, A. and Peremans, A. and Le Rille, A. and Zheng, W. Q. and Ortéga, J. M. and Glotin, F. and Prazeres, R. and Meyer, Michael and Lacoursière, J. and Nahon, L. and Gisselbrecht, M. and Morin, P. and Larzillière, M. and Marsi, M. and Taleb-Ibrahimi, A. and Couprie, M. E. and Hara, T. and Garzella, D.},
  issn         = {0909-0495},
  keyword      = {Free-electron lasers,Spectroscopy,Two-colour configurations},
  language     = {eng},
  month        = {05},
  number       = {3},
  pages        = {293--298},
  publisher    = {Wiley-Blackwell},
  series       = {Journal of Synchrotron Radiation},
  title        = {Spectroscopic techniques using synchrotron radiation and free-electron and conventional lasers},
  url          = {http://dx.doi.org/10.1107/S0909049597015392},
  volume       = {5},
  year         = {1998},
}