n exact ab initio theory of quantum transport using TDDFT and nonequilibrium Green’s functions
(2006) In ournal of Physics Conference Series 35. p.17-24- Abstract
- We present an exact ab initio theory for describing the motion of interacting electrons through nanoscopic constrictions. Our theory is based on time-dependent density functional theory (TDDFT) and nonequilibrium Green functions. We consider the system electrode-device-electrode initially contacted and in equilibrium, therefore the scheme is thermodynamically consistent. Besides the steady-state responses one can also calculate physical dynamical responses. We show that the steady-state current results from a dephasing mechanism provided the electrodes are macroscopic and the device is finite. In the d.c. case, we obtain a Landauer-like formula when the effective potential of TDDFT is uniform deep inside the electrodes.
Please use this url to cite or link to this publication:
https://lup.lub.lu.se/record/8774389
- author
- Stefanucci, Gianluca and Almbladh, Carl-Olof LU
- organization
- publishing date
- 2006
- type
- Contribution to journal
- publication status
- published
- subject
- in
- ournal of Physics Conference Series
- volume
- 35
- pages
- 17 - 24
- language
- English
- LU publication?
- yes
- id
- eed11dda-329d-4be7-b00a-b9cc8b549c8e (old id 8774389)
- date added to LUP
- 2016-04-04 13:18:35
- date last changed
- 2018-11-21 21:13:09
@article{eed11dda-329d-4be7-b00a-b9cc8b549c8e, abstract = {{We present an exact ab initio theory for describing the motion of interacting electrons through nanoscopic constrictions. Our theory is based on time-dependent density functional theory (TDDFT) and nonequilibrium Green functions. We consider the system electrode-device-electrode initially contacted and in equilibrium, therefore the scheme is thermodynamically consistent. Besides the steady-state responses one can also calculate physical dynamical responses. We show that the steady-state current results from a dephasing mechanism provided the electrodes are macroscopic and the device is finite. In the d.c. case, we obtain a Landauer-like formula when the effective potential of TDDFT is uniform deep inside the electrodes.}}, author = {{Stefanucci, Gianluca and Almbladh, Carl-Olof}}, language = {{eng}}, pages = {{17--24}}, series = {{ournal of Physics Conference Series}}, title = {{n exact ab initio theory of quantum transport using TDDFT and nonequilibrium Green’s functions}}, volume = {{35}}, year = {{2006}}, }