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Microscopic theory of light-induced ultrafast skyrmion excitation in transition metal films

Viñas Boström, Emil LU ; Rubio, Angel and Verdozzi, Claudio LU (2022) In npj Computational Materials 8(1).
Abstract

Magnetic skyrmions are topological excitations of great promise for compact and efficient memory storage. However, to interface skyrmionics with electronic devices requires efficient and reliable ways of creating and destroying such excitations. In this work, we unravel the microscopic mechanism behind ultrafast skyrmion generation by femtosecond laser pulses in transition metal thin films. We employ a theoretical approach based on a two-band electronic model, and show that by exciting the itinerant electronic subsystem with a femtosecond laser ultrafast skyrmion nucleation can occur on a 100 fs timescale. By combining numerical simulations with an analytical treatment of the strong s–d exchange limit, we identify the coupling between... (More)

Magnetic skyrmions are topological excitations of great promise for compact and efficient memory storage. However, to interface skyrmionics with electronic devices requires efficient and reliable ways of creating and destroying such excitations. In this work, we unravel the microscopic mechanism behind ultrafast skyrmion generation by femtosecond laser pulses in transition metal thin films. We employ a theoretical approach based on a two-band electronic model, and show that by exciting the itinerant electronic subsystem with a femtosecond laser ultrafast skyrmion nucleation can occur on a 100 fs timescale. By combining numerical simulations with an analytical treatment of the strong s–d exchange limit, we identify the coupling between electronic currents and the localized d-orbital spins, mediated via Rashba spin–orbit interactions among the itinerant electrons, as the microscopic and central mechanism leading to ultrafast skyrmion generation. Our results show that an explicit treatment of itinerant electron dynamics is crucial to understand optical skyrmion generation.

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publishing date
type
Contribution to journal
publication status
published
subject
in
npj Computational Materials
volume
8
issue
1
article number
62
publisher
Nature Publishing Group
external identifiers
  • scopus:85128227380
ISSN
2057-3960
DOI
10.1038/s41524-022-00735-5
language
English
LU publication?
yes
additional info
Publisher Copyright: © 2022, The Author(s).
id
8cb53b27-6995-403b-916b-b0b5922fce2e
date added to LUP
2022-04-30 22:20:39
date last changed
2024-05-16 11:09:17
@article{8cb53b27-6995-403b-916b-b0b5922fce2e,
  abstract     = {{<p>Magnetic skyrmions are topological excitations of great promise for compact and efficient memory storage. However, to interface skyrmionics with electronic devices requires efficient and reliable ways of creating and destroying such excitations. In this work, we unravel the microscopic mechanism behind ultrafast skyrmion generation by femtosecond laser pulses in transition metal thin films. We employ a theoretical approach based on a two-band electronic model, and show that by exciting the itinerant electronic subsystem with a femtosecond laser ultrafast skyrmion nucleation can occur on a 100 fs timescale. By combining numerical simulations with an analytical treatment of the strong s–d exchange limit, we identify the coupling between electronic currents and the localized d-orbital spins, mediated via Rashba spin–orbit interactions among the itinerant electrons, as the microscopic and central mechanism leading to ultrafast skyrmion generation. Our results show that an explicit treatment of itinerant electron dynamics is crucial to understand optical skyrmion generation.</p>}},
  author       = {{Viñas Boström, Emil and Rubio, Angel and Verdozzi, Claudio}},
  issn         = {{2057-3960}},
  language     = {{eng}},
  number       = {{1}},
  publisher    = {{Nature Publishing Group}},
  series       = {{npj Computational Materials}},
  title        = {{Microscopic theory of light-induced ultrafast skyrmion excitation in transition metal films}},
  url          = {{http://dx.doi.org/10.1038/s41524-022-00735-5}},
  doi          = {{10.1038/s41524-022-00735-5}},
  volume       = {{8}},
  year         = {{2022}},
}