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Multi-modal characterization of kesterite thin-film solar cells : experimental results and numerical interpretation

Saadaldin, Abdellatif ; Slyamov, Azat M. ; Stuckelberger, Michael E. ; Jørgensen, Peter S. ; Rein, Christian ; Lucas, Mariana Mar ; Ramos, Tiago ; Rodriguez-Fernandez, Angel LU ; Bernard, Dominique and Andreasen, Jens W. (2022) In Faraday Discussions 239. p.160-179
Abstract

We report a multi-modal study of the electrical, chemical and structural properties of a kesterite thin-film solar cell by combining the spatially-resolved X-ray beam induced current and fluorescence imaging techniques for the evaluation of a fully functional device on a cross-section. The data allowed the correlation of the chemical composition, defects at interfaces and inhomogeneous deposition of the layers with the local charge-collection efficiency of the device. We support our observations with Monte Carlo simulations of high-energy X-ray interactions with the semiconductor device, and finite-volume modeling of the charge-collection efficiency.

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author
; ; ; ; ; ; ; ; and
organization
publishing date
type
Contribution to journal
publication status
published
subject
in
Faraday Discussions
volume
239
pages
20 pages
publisher
Royal Society of Chemistry
external identifiers
  • pmid:35822496
  • scopus:85133879073
ISSN
1359-6640
DOI
10.1039/d2fd00044j
language
English
LU publication?
yes
id
9bead464-6853-4b8e-91d8-9bb5135db522
date added to LUP
2022-12-28 14:33:00
date last changed
2024-04-18 17:18:43
@article{9bead464-6853-4b8e-91d8-9bb5135db522,
  abstract     = {{<p>We report a multi-modal study of the electrical, chemical and structural properties of a kesterite thin-film solar cell by combining the spatially-resolved X-ray beam induced current and fluorescence imaging techniques for the evaluation of a fully functional device on a cross-section. The data allowed the correlation of the chemical composition, defects at interfaces and inhomogeneous deposition of the layers with the local charge-collection efficiency of the device. We support our observations with Monte Carlo simulations of high-energy X-ray interactions with the semiconductor device, and finite-volume modeling of the charge-collection efficiency.</p>}},
  author       = {{Saadaldin, Abdellatif and Slyamov, Azat M. and Stuckelberger, Michael E. and Jørgensen, Peter S. and Rein, Christian and Lucas, Mariana Mar and Ramos, Tiago and Rodriguez-Fernandez, Angel and Bernard, Dominique and Andreasen, Jens W.}},
  issn         = {{1359-6640}},
  language     = {{eng}},
  pages        = {{160--179}},
  publisher    = {{Royal Society of Chemistry}},
  series       = {{Faraday Discussions}},
  title        = {{Multi-modal characterization of kesterite thin-film solar cells : experimental results and numerical interpretation}},
  url          = {{http://dx.doi.org/10.1039/d2fd00044j}},
  doi          = {{10.1039/d2fd00044j}},
  volume       = {{239}},
  year         = {{2022}},
}