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Broad spectral photocurrent enhancement in Au-decorated CdSe nanowires

Chakraborty, Ritun ; Greullet, Fanny ; George, Chandramohan ; Baranov, Dmitry LU orcid ; Di Fabrizio, Enzo and Krahne, Roman (2013) In Nanoscale 5(12). p.5334-5340
Abstract

Metal-semiconductor hybrid nanostructures promise improved photoconductive performance due to plasmonic properties of the metal portions and intrinsic electric fields at the metal-semiconductor interface that possibly enhance charge separation. Here we report gold decorated CdSe nanowires as a novel functional material and investigate the influence of gold decoration on the lateral facets on the photoconductive properties. Gold decorated nanowires show typically an at least ten-fold higher photocurrent as compared to their bare counterparts. Interestingly, the photocurrent enhancement is wavelength independent, although the plasmon resonance related to the gold particles appears in the absorption spectra. Our experiments show that light... (More)

Metal-semiconductor hybrid nanostructures promise improved photoconductive performance due to plasmonic properties of the metal portions and intrinsic electric fields at the metal-semiconductor interface that possibly enhance charge separation. Here we report gold decorated CdSe nanowires as a novel functional material and investigate the influence of gold decoration on the lateral facets on the photoconductive properties. Gold decorated nanowires show typically an at least ten-fold higher photocurrent as compared to their bare counterparts. Interestingly, the photocurrent enhancement is wavelength independent, although the plasmon resonance related to the gold particles appears in the absorption spectra. Our experiments show that light scattering and Schottky fields associated with the metal-semiconductor interface are at the origin of the photocurrent enhancement.

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Please use this url to cite or link to this publication:
author
; ; ; ; and
publishing date
type
Contribution to journal
publication status
published
in
Nanoscale
volume
5
issue
12
pages
7 pages
publisher
Royal Society of Chemistry
external identifiers
  • scopus:84878745861
ISSN
2040-3364
DOI
10.1039/c3nr00752a
language
English
LU publication?
no
id
9fc69293-6cee-4c6b-b23c-9a8d5eb913f3
date added to LUP
2023-01-18 09:34:15
date last changed
2023-02-14 10:35:16
@article{9fc69293-6cee-4c6b-b23c-9a8d5eb913f3,
  abstract     = {{<p>Metal-semiconductor hybrid nanostructures promise improved photoconductive performance due to plasmonic properties of the metal portions and intrinsic electric fields at the metal-semiconductor interface that possibly enhance charge separation. Here we report gold decorated CdSe nanowires as a novel functional material and investigate the influence of gold decoration on the lateral facets on the photoconductive properties. Gold decorated nanowires show typically an at least ten-fold higher photocurrent as compared to their bare counterparts. Interestingly, the photocurrent enhancement is wavelength independent, although the plasmon resonance related to the gold particles appears in the absorption spectra. Our experiments show that light scattering and Schottky fields associated with the metal-semiconductor interface are at the origin of the photocurrent enhancement.</p>}},
  author       = {{Chakraborty, Ritun and Greullet, Fanny and George, Chandramohan and Baranov, Dmitry and Di Fabrizio, Enzo and Krahne, Roman}},
  issn         = {{2040-3364}},
  language     = {{eng}},
  month        = {{06}},
  number       = {{12}},
  pages        = {{5334--5340}},
  publisher    = {{Royal Society of Chemistry}},
  series       = {{Nanoscale}},
  title        = {{Broad spectral photocurrent enhancement in Au-decorated CdSe nanowires}},
  url          = {{http://dx.doi.org/10.1039/c3nr00752a}},
  doi          = {{10.1039/c3nr00752a}},
  volume       = {{5}},
  year         = {{2013}},
}