Interferometric quantum control (IQC) by fs/ns rotational coherent anti-Stokes Raman spectroscopy (RCARS)
Raveesh, Meena LU ; Dominguez, Armand LU ; Linne, Mark ; Bood, Joakim LU and Hosseinnia, Ali LU
(2023)
In Optics Express
31(23).
p.38064-38076
- Abstract
A new rotational coherent anti-Stokes Raman spectroscopy (RCARS) concept based on interferometric quantum control (IQC) is demonstrated. Two wavepackets originating from pure rotational states are created by a femtosecond stimulated rotational Raman interaction. The two Raman responses are instantly probed by a single-mode ns pulse generating two interfering RCARS polarizations. The resulting signal is an IQC-RCARS spectrum detected by a streak camera. Here we demonstrate IQC-interferograms of N2 by varying the temporal separation between the two fs pulses within a full rotational revival period, as well as signal amplification and selective detection of nuclear-spin isomers at room conditions and inside a flame.
Please use this url to cite or link to this publication:
https://lup.lub.lu.se/record/b1e162ed-21e6-4283-a945-982093511fbe
- author
- Raveesh, Meena
LU
; Dominguez, Armand
LU
; Linne, Mark
; Bood, Joakim
LU
and Hosseinnia, Ali
LU
- organization
- publishing date
- 2023-11-06
- type
- Contribution to journal
- publication status
- published
- subject
- in
- Optics Express
- volume
- 31
- issue
- 23
- pages
- 13 pages
- publisher
- Optical Society of America
- external identifiers
-
- pmid:38017923
- scopus:85177977238
- ISSN
- 1094-4087
- DOI
- 10.1364/OE.498169
- language
- English
- LU publication?
- yes
- id
- b1e162ed-21e6-4283-a945-982093511fbe
- date added to LUP
- 2023-12-29 13:45:41
- date last changed
- 2024-12-22 21:44:31
@article{b1e162ed-21e6-4283-a945-982093511fbe,
abstract = {{<p>A new rotational coherent anti-Stokes Raman spectroscopy (RCARS) concept based on interferometric quantum control (IQC) is demonstrated. Two wavepackets originating from pure rotational states are created by a femtosecond stimulated rotational Raman interaction. The two Raman responses are instantly probed by a single-mode ns pulse generating two interfering RCARS polarizations. The resulting signal is an IQC-RCARS spectrum detected by a streak camera. Here we demonstrate IQC-interferograms of N<sub>2</sub> by varying the temporal separation between the two fs pulses within a full rotational revival period, as well as signal amplification and selective detection of nuclear-spin isomers at room conditions and inside a flame.</p>}},
author = {{Raveesh, Meena and Dominguez, Armand and Linne, Mark and Bood, Joakim and Hosseinnia, Ali}},
issn = {{1094-4087}},
language = {{eng}},
month = {{11}},
number = {{23}},
pages = {{38064--38076}},
publisher = {{Optical Society of America}},
series = {{Optics Express}},
title = {{Interferometric quantum control (IQC) by fs/ns rotational coherent anti-Stokes Raman spectroscopy (RCARS)}},
url = {{http://dx.doi.org/10.1364/OE.498169}},
doi = {{10.1364/OE.498169}},
volume = {{31}},
year = {{2023}},
}