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Interpretation and Utility of the Moments of Small-Angle X-Ray Scattering Distributions

Modregger, Peter ; Kagias, Matias LU orcid ; Irvine, Sarah C. ; Brönnimann, Rolf ; Jefimovs, Konstantins ; Endrizzi, Marco and Olivo, Alessandro (2017) In Physical Review Letters 118(26).
Abstract

Small angle X-ray scattering has been proven to be a valuable method for accessing structural information below the spatial resolution limit implied by direct imaging. Here, we theoretically derive the relation that links the subpixel differential phase signal provided by the sample to the moments of scattering distributions accessible by refraction sensitive X-ray imaging techniques. As an important special case we explain the scatter or dark-field contrast in terms of the sample's phase signal. Further, we establish that, for binary phase objects, the nth moment scales with the difference of the refractive index decrement to the power of n. Finally, we experimentally demonstrate the utility of the moments by quantitatively determining... (More)

Small angle X-ray scattering has been proven to be a valuable method for accessing structural information below the spatial resolution limit implied by direct imaging. Here, we theoretically derive the relation that links the subpixel differential phase signal provided by the sample to the moments of scattering distributions accessible by refraction sensitive X-ray imaging techniques. As an important special case we explain the scatter or dark-field contrast in terms of the sample's phase signal. Further, we establish that, for binary phase objects, the nth moment scales with the difference of the refractive index decrement to the power of n. Finally, we experimentally demonstrate the utility of the moments by quantitatively determining the particle sizes of a range of powders with a laboratory-based setup.

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author
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publishing date
type
Contribution to journal
publication status
published
subject
in
Physical Review Letters
volume
118
issue
26
article number
265501
publisher
American Physical Society
external identifiers
  • scopus:85021732686
  • pmid:28707948
ISSN
0031-9007
DOI
10.1103/PhysRevLett.118.265501
language
English
LU publication?
no
additional info
Publisher Copyright: © 2017 authors.
id
bdbb691c-2b6f-42e9-80f5-5374f06168fa
date added to LUP
2023-11-27 09:03:51
date last changed
2024-03-13 16:05:51
@article{bdbb691c-2b6f-42e9-80f5-5374f06168fa,
  abstract     = {{<p>Small angle X-ray scattering has been proven to be a valuable method for accessing structural information below the spatial resolution limit implied by direct imaging. Here, we theoretically derive the relation that links the subpixel differential phase signal provided by the sample to the moments of scattering distributions accessible by refraction sensitive X-ray imaging techniques. As an important special case we explain the scatter or dark-field contrast in terms of the sample's phase signal. Further, we establish that, for binary phase objects, the nth moment scales with the difference of the refractive index decrement to the power of n. Finally, we experimentally demonstrate the utility of the moments by quantitatively determining the particle sizes of a range of powders with a laboratory-based setup.</p>}},
  author       = {{Modregger, Peter and Kagias, Matias and Irvine, Sarah C. and Brönnimann, Rolf and Jefimovs, Konstantins and Endrizzi, Marco and Olivo, Alessandro}},
  issn         = {{0031-9007}},
  language     = {{eng}},
  month        = {{06}},
  number       = {{26}},
  publisher    = {{American Physical Society}},
  series       = {{Physical Review Letters}},
  title        = {{Interpretation and Utility of the Moments of Small-Angle X-Ray Scattering Distributions}},
  url          = {{http://dx.doi.org/10.1103/PhysRevLett.118.265501}},
  doi          = {{10.1103/PhysRevLett.118.265501}},
  volume       = {{118}},
  year         = {{2017}},
}