CysK2 from Mycobacterium tuberculosis is an O-phospho-L-serine-dependent S-sulfocysteine synthase
(2014) In Journal of Bacteriology 196(19). p.3410-3420- Abstract
Mycobacterium tuberculosis is dependent on cysteine biosynthesis, and reduced sulfur compounds such as mycothiol synthesized from cysteine serve in first-line defense mechanisms against oxidative stress imposed by macrophages. Two biosynthetic routes to L-cysteine, each with its own specific cysteine synthase (CysK1 and CysM), have been described in M. tuberculosis, but the function of a third putative sulfhydrylase in this pathogen, CysK2, has remained elusive. We present biochemical and biophysical evidence that CysK2 is an S-sulfocysteine synthase, utilizing O-phosphoserine (OPS) and thiosulfate as substrates. The enzyme uses a mechanism via a central aminoacrylate intermediate that is similar to that of other members of this... (More)
Mycobacterium tuberculosis is dependent on cysteine biosynthesis, and reduced sulfur compounds such as mycothiol synthesized from cysteine serve in first-line defense mechanisms against oxidative stress imposed by macrophages. Two biosynthetic routes to L-cysteine, each with its own specific cysteine synthase (CysK1 and CysM), have been described in M. tuberculosis, but the function of a third putative sulfhydrylase in this pathogen, CysK2, has remained elusive. We present biochemical and biophysical evidence that CysK2 is an S-sulfocysteine synthase, utilizing O-phosphoserine (OPS) and thiosulfate as substrates. The enzyme uses a mechanism via a central aminoacrylate intermediate that is similar to that of other members of this pyridoxal phosphate-dependent enzyme family. The apparent second-order rate of the first half-reaction with OPS was determined as kmax/Ks=(3.97×103)±619M-1 s-1, which compares well to the OPS-specific mycobacterial cysteine synthase CysM with a kmax/Ks of (1.34×103)±48.2. Notably, CysK2 does not utilize thiocarboxylated CysO as a sulfur donor but accepts thiosulfate and sulfide as donor substrates. The specificity constant kcat/Km for thiosulfate is 40-fold higher than for sulfide, suggesting an annotation as S-sulfocysteine synthase. Mycobacterial CysK2 thus provides a third metabolic route to cysteine, either directly using sulfide as donor or indirectly via S-sulfocysteine. Hypothetically, S-sulfocysteine could also act as a signaling molecule triggering additional responses in redox defense in the pathogen upon exposure to reactive oxygen species during dormancy.
(Less)
- author
- Steiner, Eva Maria
LU
; Bo¨th, Dominic ; Lo¨ssl, Philip ; Vilaplana, Francisco ; Schnell, Robert and Schneider, Gunter
- publishing date
- 2014
- type
- Contribution to journal
- publication status
- published
- in
- Journal of Bacteriology
- volume
- 196
- issue
- 19
- pages
- 3410 - 3420
- publisher
- American Society for Microbiology
- external identifiers
-
- pmid:25022854
- scopus:84907016411
- ISSN
- 0021-9193
- DOI
- 10.1128/JB.01851-14
- language
- English
- LU publication?
- no
- additional info
- Publisher Copyright: © 2014, American Society for Microbiology.
- id
- cc5747e3-fc3f-4dda-9980-32a596f0e766
- date added to LUP
- 2024-06-24 11:28:12
- date last changed
- 2025-01-07 06:35:12
@article{cc5747e3-fc3f-4dda-9980-32a596f0e766, abstract = {{<p>Mycobacterium tuberculosis is dependent on cysteine biosynthesis, and reduced sulfur compounds such as mycothiol synthesized from cysteine serve in first-line defense mechanisms against oxidative stress imposed by macrophages. Two biosynthetic routes to L-cysteine, each with its own specific cysteine synthase (CysK1 and CysM), have been described in M. tuberculosis, but the function of a third putative sulfhydrylase in this pathogen, CysK2, has remained elusive. We present biochemical and biophysical evidence that CysK2 is an S-sulfocysteine synthase, utilizing O-phosphoserine (OPS) and thiosulfate as substrates. The enzyme uses a mechanism via a central aminoacrylate intermediate that is similar to that of other members of this pyridoxal phosphate-dependent enzyme family. The apparent second-order rate of the first half-reaction with OPS was determined as k<sub>max</sub>/K<sub>s</sub>=(3.97×10<sup>3</sup>)±619M<sup>-1</sup> s<sup>-1</sup>, which compares well to the OPS-specific mycobacterial cysteine synthase CysM with a k<sub>max</sub>/K<sub>s</sub> of (1.34×10<sup>3</sup>)±48.2. Notably, CysK2 does not utilize thiocarboxylated CysO as a sulfur donor but accepts thiosulfate and sulfide as donor substrates. The specificity constant k<sub>cat</sub>/K<sub>m</sub> for thiosulfate is 40-fold higher than for sulfide, suggesting an annotation as S-sulfocysteine synthase. Mycobacterial CysK2 thus provides a third metabolic route to cysteine, either directly using sulfide as donor or indirectly via S-sulfocysteine. Hypothetically, S-sulfocysteine could also act as a signaling molecule triggering additional responses in redox defense in the pathogen upon exposure to reactive oxygen species during dormancy.</p>}}, author = {{Steiner, Eva Maria and Bo¨th, Dominic and Lo¨ssl, Philip and Vilaplana, Francisco and Schnell, Robert and Schneider, Gunter}}, issn = {{0021-9193}}, language = {{eng}}, number = {{19}}, pages = {{3410--3420}}, publisher = {{American Society for Microbiology}}, series = {{Journal of Bacteriology}}, title = {{CysK2 from Mycobacterium tuberculosis is an O-phospho-L-serine-dependent S-sulfocysteine synthase}}, url = {{http://dx.doi.org/10.1128/JB.01851-14}}, doi = {{10.1128/JB.01851-14}}, volume = {{196}}, year = {{2014}}, }