Photon pumping, photodissociation and dissipation at interplay for the fluorescence of a molecule in a cavity
(2023) In SciPost Physics 15(4).- Abstract
We introduce a model description of a diatomic molecule in an optical cavity, with pump and fluorescent fields, and electron and nuclear motion are treated on equal footing and exactly. The model accounts for several optical response temporal scenarios: A Mollow spectrum hindered by electron correlations, a competition of harmonic generation and molecular dissociation, a dependence of fluorescence on photon pumping rate and dissipation. It is thus a general and flexible template for insight into experiments where quantum photon confinement, leakage, nuclear motion and electronic correlations are at interplay.
Please use this url to cite or link to this publication:
https://lup.lub.lu.se/record/d118424e-b210-40e5-b1dd-4c5ad452fccf
- author
- Gopalakrishna, Megha LU ; Boström, Emil Viñas LU and Verdozzi, Claudio LU
- organization
- publishing date
- 2023-10
- type
- Contribution to journal
- publication status
- published
- subject
- in
- SciPost Physics
- volume
- 15
- issue
- 4
- article number
- 138
- publisher
- SciPost
- external identifiers
-
- scopus:85178045449
- ISSN
- 2542-4653
- DOI
- 10.21468/SciPostPhys.15.4.138
- language
- English
- LU publication?
- yes
- additional info
- Funding Information: Funding information M.G. and C.V. acknowledge support from the Swedish Research Council (grants number 2017-03945 and 2022-04486). Publisher Copyright: Copyright M. Gopalakrishna et al.
- id
- d118424e-b210-40e5-b1dd-4c5ad452fccf
- date added to LUP
- 2024-01-05 09:29:14
- date last changed
- 2024-02-02 07:24:51
@article{d118424e-b210-40e5-b1dd-4c5ad452fccf, abstract = {{<p>We introduce a model description of a diatomic molecule in an optical cavity, with pump and fluorescent fields, and electron and nuclear motion are treated on equal footing and exactly. The model accounts for several optical response temporal scenarios: A Mollow spectrum hindered by electron correlations, a competition of harmonic generation and molecular dissociation, a dependence of fluorescence on photon pumping rate and dissipation. It is thus a general and flexible template for insight into experiments where quantum photon confinement, leakage, nuclear motion and electronic correlations are at interplay.</p>}}, author = {{Gopalakrishna, Megha and Boström, Emil Viñas and Verdozzi, Claudio}}, issn = {{2542-4653}}, language = {{eng}}, number = {{4}}, publisher = {{SciPost}}, series = {{SciPost Physics}}, title = {{Photon pumping, photodissociation and dissipation at interplay for the fluorescence of a molecule in a cavity}}, url = {{http://dx.doi.org/10.21468/SciPostPhys.15.4.138}}, doi = {{10.21468/SciPostPhys.15.4.138}}, volume = {{15}}, year = {{2023}}, }