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Epsilon-Near-Zero Substrate Engineering for Ultrathin-Film Perfect Absorbers

Rensberg, Jura ; Zhou, You ; Richter, Steffen LU ; Wan, Chenghao ; Zhang, Shuyan ; Schöppe, Philipp ; Schmidt-Grund, Rüdiger ; Ramanathan, Shriram ; Capasso, Federico and Kats, Mikhail A. , et al. (2017) In Physical Review Applied 8(1).
Abstract

Efficient suppression of reflection is a key requirement for perfect absorption of light. Recently, it has been shown that reflection can be effectively suppressed utilizing a single ultrathin film deposited on metals or polar materials featuring phonon resonances. The wavelength at which reflection can be fully suppressed is primarily determined by the nature of these substrates and is pinned to particular values near plasma or phonon resonances - the former typically in the ultraviolet or visible and the latter in the infrared. Here, we explicitly identify the required optical properties of films and substrates for the design of absorbing antireflection coatings based on ultrathin films. We find that completely suppressed reflection... (More)

Efficient suppression of reflection is a key requirement for perfect absorption of light. Recently, it has been shown that reflection can be effectively suppressed utilizing a single ultrathin film deposited on metals or polar materials featuring phonon resonances. The wavelength at which reflection can be fully suppressed is primarily determined by the nature of these substrates and is pinned to particular values near plasma or phonon resonances - the former typically in the ultraviolet or visible and the latter in the infrared. Here, we explicitly identify the required optical properties of films and substrates for the design of absorbing antireflection coatings based on ultrathin films. We find that completely suppressed reflection using films with thicknesses much smaller than the wavelength of light occurs within a spectral region where the real part of the refractive index of the substrate is n1, which is characteristic of materials with permittivity close to zero. We experimentally verify this condition by using an ultrathin vanadium dioxide film with dynamically tunable optical properties on several epsilon-near-zero materials, including aluminum-doped zinc oxide. By tailoring the plasma frequency of the aluminum-doped zinc oxide, we are able to tune the epsilon-near-zero point, thus achieving suppressed reflection and near-perfect absorption at wavelengths that continuously span the near-infrared and long-wave midinfrared ranges.

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publishing date
type
Contribution to journal
publication status
published
in
Physical Review Applied
volume
8
issue
1
article number
014009
publisher
American Physical Society
external identifiers
  • scopus:85024495546
ISSN
2331-7019
DOI
10.1103/PhysRevApplied.8.014009
language
English
LU publication?
no
additional info
Publisher Copyright: © 2017 American Physical Society.
id
eed19add-3a7b-4aba-b60b-47b8f62a97a1
date added to LUP
2022-04-19 14:49:45
date last changed
2022-04-25 16:23:40
@article{eed19add-3a7b-4aba-b60b-47b8f62a97a1,
  abstract     = {{<p>Efficient suppression of reflection is a key requirement for perfect absorption of light. Recently, it has been shown that reflection can be effectively suppressed utilizing a single ultrathin film deposited on metals or polar materials featuring phonon resonances. The wavelength at which reflection can be fully suppressed is primarily determined by the nature of these substrates and is pinned to particular values near plasma or phonon resonances - the former typically in the ultraviolet or visible and the latter in the infrared. Here, we explicitly identify the required optical properties of films and substrates for the design of absorbing antireflection coatings based on ultrathin films. We find that completely suppressed reflection using films with thicknesses much smaller than the wavelength of light occurs within a spectral region where the real part of the refractive index of the substrate is n1, which is characteristic of materials with permittivity close to zero. We experimentally verify this condition by using an ultrathin vanadium dioxide film with dynamically tunable optical properties on several epsilon-near-zero materials, including aluminum-doped zinc oxide. By tailoring the plasma frequency of the aluminum-doped zinc oxide, we are able to tune the epsilon-near-zero point, thus achieving suppressed reflection and near-perfect absorption at wavelengths that continuously span the near-infrared and long-wave midinfrared ranges.</p>}},
  author       = {{Rensberg, Jura and Zhou, You and Richter, Steffen and Wan, Chenghao and Zhang, Shuyan and Schöppe, Philipp and Schmidt-Grund, Rüdiger and Ramanathan, Shriram and Capasso, Federico and Kats, Mikhail A. and Ronning, Carsten}},
  issn         = {{2331-7019}},
  language     = {{eng}},
  month        = {{07}},
  number       = {{1}},
  publisher    = {{American Physical Society}},
  series       = {{Physical Review Applied}},
  title        = {{Epsilon-Near-Zero Substrate Engineering for Ultrathin-Film Perfect Absorbers}},
  url          = {{http://dx.doi.org/10.1103/PhysRevApplied.8.014009}},
  doi          = {{10.1103/PhysRevApplied.8.014009}},
  volume       = {{8}},
  year         = {{2017}},
}