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Systematic experimental study for optimized hydrogen production of Ni/CeO2 prepared by incipient wetness impregnation technique

Li, Shian LU ; Shen, Qiuwan LU and Sunden, Bengt LU (2020) In Journal of Ceramic Processing Research 21(2). p.263-268
Abstract

In this present work, different supports (CeO2/ZrO2) and different Ni contents based catalysts were prepared by incipient wetness impregnation method and tested in the methane steam reforming (MSR) reaction. The prepared catalysts were characterized by X-ray diffraction (XRD) and scanning electron microscope (SEM). The XRD analysis confirmed the prepared Ni/CeO2 samples have a pure crystal structure. In the catalytic tests, the effects of reactivity temperature, different support, Ni loading content and the gas hourly space velocity (GHSV) on hydrogen production performance were investigated systematically. The results showed that the optimal reaction conditions for MSR by Ni/CeO2 catalyst... (More)

In this present work, different supports (CeO2/ZrO2) and different Ni contents based catalysts were prepared by incipient wetness impregnation method and tested in the methane steam reforming (MSR) reaction. The prepared catalysts were characterized by X-ray diffraction (XRD) and scanning electron microscope (SEM). The XRD analysis confirmed the prepared Ni/CeO2 samples have a pure crystal structure. In the catalytic tests, the effects of reactivity temperature, different support, Ni loading content and the gas hourly space velocity (GHSV) on hydrogen production performance were investigated systematically. The results showed that the optimal reaction conditions for MSR by Ni/CeO2 catalyst were as follows: 10 wt % Ni/CeO2, 750oC, 1500 h−1. The stability test for 12 h at 750oC indicated that the chosen Ni/CeO2 catalyst had excellent thermal stability.

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Please use this url to cite or link to this publication:
author
; and
organization
publishing date
type
Contribution to journal
publication status
published
subject
keywords
CeO, Hydrogen, Ni, Steam reforming, Support
in
Journal of Ceramic Processing Research
volume
21
issue
2
pages
6 pages
publisher
Hanyang University
external identifiers
  • scopus:85085118736
ISSN
1229-9162
DOI
10.36410/jcpr.2020.21.2.263
language
English
LU publication?
yes
id
f29928ae-7848-465f-90d9-b8cbaacdfa1e
date added to LUP
2020-06-24 13:27:33
date last changed
2023-11-05 19:09:45
@article{f29928ae-7848-465f-90d9-b8cbaacdfa1e,
  abstract     = {{<p>In this present work, different supports (CeO<sub>2</sub>/ZrO<sub>2</sub>) and different Ni contents based catalysts were prepared by incipient wetness impregnation method and tested in the methane steam reforming (MSR) reaction. The prepared catalysts were characterized by X-ray diffraction (XRD) and scanning electron microscope (SEM). The XRD analysis confirmed the prepared Ni/CeO<sub>2</sub> samples have a pure crystal structure. In the catalytic tests, the effects of reactivity temperature, different support, Ni loading content and the gas hourly space velocity (GHSV) on hydrogen production performance were investigated systematically. The results showed that the optimal reaction conditions for MSR by Ni/CeO<sub>2</sub> catalyst were as follows: 10 wt % Ni/CeO<sub>2</sub>, 750<sup>o</sup>C, 1500 h<sup>−1</sup>. The stability test for 12 h at 750<sup>o</sup>C indicated that the chosen Ni/CeO<sub>2</sub> catalyst had excellent thermal stability.</p>}},
  author       = {{Li, Shian and Shen, Qiuwan and Sunden, Bengt}},
  issn         = {{1229-9162}},
  keywords     = {{CeO; Hydrogen; Ni; Steam reforming; Support}},
  language     = {{eng}},
  number       = {{2}},
  pages        = {{263--268}},
  publisher    = {{Hanyang University}},
  series       = {{Journal of Ceramic Processing Research}},
  title        = {{Systematic experimental study for optimized hydrogen production of Ni/CeO<sub>2</sub> prepared by incipient wetness impregnation technique}},
  url          = {{http://dx.doi.org/10.36410/jcpr.2020.21.2.263}},
  doi          = {{10.36410/jcpr.2020.21.2.263}},
  volume       = {{21}},
  year         = {{2020}},
}