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Water oxidation catalyzed by molecular Di- and nonanuclear Fe complexes : Importance of a proper ligand framework

Das, Biswanath LU ; Lee, Bao Lin; Karlsson, Erik A.; Åkermark, Torbjörn; Shatskiy, Andrey; Demeshko, Serhiy; Liao, Rong-Zhen; Laine, Tanja M.; Haukka, Matti and Zeglio, Erica, et al. (2016) In Dalton Transactions 45(34). p.13289-13293
Abstract

The synthesis of two molecular iron complexes, a dinuclear iron(III,III) complex and a nonanuclear iron complex, based on the dinucleating ligand 2,2'-(2-hydroxy-5-methyl-1,3-phenylene)bis(1H-benzo[d]imidazole-4-carboxylic acid) is described. The two iron complexes were found to drive the oxidation of water by the oneelectron oxidant [Ru(bpy)3]3+.

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organization
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type
Contribution to journal
publication status
published
subject
in
Dalton Transactions
volume
45
issue
34
pages
5 pages
publisher
Royal Society of Chemistry
external identifiers
  • scopus:84983638449
  • wos:000382144300004
ISSN
1477-9226
DOI
10.1039/c6dt01554a
language
English
LU publication?
yes
id
f6d1f792-8675-40dc-8a67-a480611b2485
date added to LUP
2017-02-07 11:21:11
date last changed
2017-09-24 05:06:53
@article{f6d1f792-8675-40dc-8a67-a480611b2485,
  abstract     = {<p>The synthesis of two molecular iron complexes, a dinuclear iron(III,III) complex and a nonanuclear iron complex, based on the dinucleating ligand 2,2'-(2-hydroxy-5-methyl-1,3-phenylene)bis(1H-benzo[d]imidazole-4-carboxylic acid) is described. The two iron complexes were found to drive the oxidation of water by the oneelectron oxidant [Ru(bpy)<sub>3</sub>]<sup>3+</sup>.</p>},
  author       = {Das, Biswanath and Lee, Bao Lin and Karlsson, Erik A. and Åkermark, Torbjörn and Shatskiy, Andrey and Demeshko, Serhiy and Liao, Rong-Zhen and Laine, Tanja M. and Haukka, Matti and Zeglio, Erica and Abdel-Magied, Ahmed F. and Siegbahn, Per E M and Meyer, Franc and Kärkäs, Markus D. and Johnston, Eric V. and Nordlander, Ebbe and Åkermark, Björn},
  issn         = {1477-9226},
  language     = {eng},
  number       = {34},
  pages        = {13289--13293},
  publisher    = {Royal Society of Chemistry},
  series       = {Dalton Transactions},
  title        = {Water oxidation catalyzed by molecular Di- and nonanuclear Fe complexes : Importance of a proper ligand framework},
  url          = {http://dx.doi.org/10.1039/c6dt01554a},
  volume       = {45},
  year         = {2016},
}