Role of Thermal Equilibrium Dynamics in Atomic Motion during Nonthermal Laser-Induced Melting
(2020) In Physical Review Letters 124(10).- Abstract
This study shows that initial atomic velocities as given by thermodynamics play an important role in the dynamics of phase transitions. We tracked the atomic motion during nonthermal laser-induced melting of InSb at different initial temperatures. The ultrafast atomic motion following bond breaking can in general be governed by two mechanisms: the random velocity of each atom at the time of bond breaking (inertial model), and the forces acting on the atoms after bond breaking. The melting dynamics was found to follow the inertial model over a wide temperature range.
Please use this url to cite or link to this publication:
https://lup.lub.lu.se/record/f7fb1329-5b68-4342-96dc-a86b16e0a93c
- author
- Wang, Xiaocui LU ; Ekström, J C ; Bengtsson, Å U J LU ; Jarnac, A LU ; Jurgilaitis, A LU ; Pham, Van-Thai LU ; Kroon, D LU ; Enquist, H LU and Larsson, J LU
- organization
- publishing date
- 2020-03-13
- type
- Contribution to journal
- publication status
- published
- subject
- in
- Physical Review Letters
- volume
- 124
- issue
- 10
- article number
- 105701
- publisher
- American Physical Society
- external identifiers
-
- pmid:32216426
- scopus:85082508306
- ISSN
- 1079-7114
- DOI
- 10.1103/PhysRevLett.124.105701
- language
- English
- LU publication?
- yes
- id
- f7fb1329-5b68-4342-96dc-a86b16e0a93c
- date added to LUP
- 2020-04-01 22:43:53
- date last changed
- 2024-05-01 07:22:13
@article{f7fb1329-5b68-4342-96dc-a86b16e0a93c, abstract = {{<p>This study shows that initial atomic velocities as given by thermodynamics play an important role in the dynamics of phase transitions. We tracked the atomic motion during nonthermal laser-induced melting of InSb at different initial temperatures. The ultrafast atomic motion following bond breaking can in general be governed by two mechanisms: the random velocity of each atom at the time of bond breaking (inertial model), and the forces acting on the atoms after bond breaking. The melting dynamics was found to follow the inertial model over a wide temperature range.</p>}}, author = {{Wang, Xiaocui and Ekström, J C and Bengtsson, Å U J and Jarnac, A and Jurgilaitis, A and Pham, Van-Thai and Kroon, D and Enquist, H and Larsson, J}}, issn = {{1079-7114}}, language = {{eng}}, month = {{03}}, number = {{10}}, publisher = {{American Physical Society}}, series = {{Physical Review Letters}}, title = {{Role of Thermal Equilibrium Dynamics in Atomic Motion during Nonthermal Laser-Induced Melting}}, url = {{http://dx.doi.org/10.1103/PhysRevLett.124.105701}}, doi = {{10.1103/PhysRevLett.124.105701}}, volume = {{124}}, year = {{2020}}, }