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Role of Thermal Equilibrium Dynamics in Atomic Motion during Nonthermal Laser-Induced Melting

Wang, Xiaocui LU ; Ekström, J C ; Bengtsson, Å U J LU ; Jarnac, A LU ; Jurgilaitis, A LU ; Pham, Van-Thai LU ; Kroon, D LU ; Enquist, H LU orcid and Larsson, J LU orcid (2020) In Physical Review Letters 124(10).
Abstract

This study shows that initial atomic velocities as given by thermodynamics play an important role in the dynamics of phase transitions. We tracked the atomic motion during nonthermal laser-induced melting of InSb at different initial temperatures. The ultrafast atomic motion following bond breaking can in general be governed by two mechanisms: the random velocity of each atom at the time of bond breaking (inertial model), and the forces acting on the atoms after bond breaking. The melting dynamics was found to follow the inertial model over a wide temperature range.

Please use this url to cite or link to this publication:
author
; ; ; ; ; ; ; and
organization
publishing date
type
Contribution to journal
publication status
published
subject
in
Physical Review Letters
volume
124
issue
10
article number
105701
publisher
American Physical Society
external identifiers
  • pmid:32216426
  • scopus:85082508306
ISSN
1079-7114
DOI
10.1103/PhysRevLett.124.105701
language
English
LU publication?
yes
id
f7fb1329-5b68-4342-96dc-a86b16e0a93c
date added to LUP
2020-04-01 22:43:53
date last changed
2024-05-01 07:22:13
@article{f7fb1329-5b68-4342-96dc-a86b16e0a93c,
  abstract     = {{<p>This study shows that initial atomic velocities as given by thermodynamics play an important role in the dynamics of phase transitions. We tracked the atomic motion during nonthermal laser-induced melting of InSb at different initial temperatures. The ultrafast atomic motion following bond breaking can in general be governed by two mechanisms: the random velocity of each atom at the time of bond breaking (inertial model), and the forces acting on the atoms after bond breaking. The melting dynamics was found to follow the inertial model over a wide temperature range.</p>}},
  author       = {{Wang, Xiaocui and Ekström, J C and Bengtsson, Å U J and Jarnac, A and Jurgilaitis, A and Pham, Van-Thai and Kroon, D and Enquist, H and Larsson, J}},
  issn         = {{1079-7114}},
  language     = {{eng}},
  month        = {{03}},
  number       = {{10}},
  publisher    = {{American Physical Society}},
  series       = {{Physical Review Letters}},
  title        = {{Role of Thermal Equilibrium Dynamics in Atomic Motion during Nonthermal Laser-Induced Melting}},
  url          = {{http://dx.doi.org/10.1103/PhysRevLett.124.105701}},
  doi          = {{10.1103/PhysRevLett.124.105701}},
  volume       = {{124}},
  year         = {{2020}},
}