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Contributions of dust and biomass burning to aerosols at a Colorado mountain-top site

Hallar, A. G. ; Petersen, R. LU ; Andrews, Elisabeth ; Michalsky, J. ; McCubbin, I. B. and Ogren, J. A. (2015) In Atmospheric Chemistry and Physics 15(23). p.13665-13679
Abstract

Visible Multifilter Rotating Shadowband Radiometer (vis-MFRSR) data were collected at Storm Peak Laboratory (SPL), a mountain-top facility in northwest Colorado, from 1999 to 2011 and in 2013. From 2011 to 2014, in situ measurements of aerosol light scattering were also obtained. Using these data sets together, the seasonal impact of dust and biomass burning is considered for the western USA. Analysis indicates that the median contributions to spring and summer aerosol optical depth (AOD) from dust and biomass-burning aerosols across the data set are comparable. The mean AOD is slightly greater in the summer, with significantly more frequent and short-duration high AOD measurements due to biomass-burning episodes than in the spring. The... (More)

Visible Multifilter Rotating Shadowband Radiometer (vis-MFRSR) data were collected at Storm Peak Laboratory (SPL), a mountain-top facility in northwest Colorado, from 1999 to 2011 and in 2013. From 2011 to 2014, in situ measurements of aerosol light scattering were also obtained. Using these data sets together, the seasonal impact of dust and biomass burning is considered for the western USA. Analysis indicates that the median contributions to spring and summer aerosol optical depth (AOD) from dust and biomass-burning aerosols across the data set are comparable. The mean AOD is slightly greater in the summer, with significantly more frequent and short-duration high AOD measurements due to biomass-burning episodes than in the spring. The Ångström exponent showed a significant increase in the summer for both the in situ and vis-MFRSR data, suggesting an increase in combustion aerosols. Spring dust events are less distinguishable in the in situ data than the column measurement, suggesting that a significant amount of dust may be found above the elevation of SPL, 3220 m a.s.l. Twenty-two known case studies of intercontinental dust, regional dust, and biomass-burning events were investigated. These events were found to follow a similar pattern, in both aerosol loading and Ångström exponent, as the seasonal mean signal in both the vis-MFRSR and ground-based nephelometer. This data set highlights the wide-scale implications of a warmer, drier climate on visibility in the western USA.

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publishing date
type
Contribution to journal
publication status
published
subject
in
Atmospheric Chemistry and Physics
volume
15
issue
23
pages
15 pages
publisher
Copernicus GmbH
external identifiers
  • scopus:84949637364
ISSN
1680-7316
DOI
10.5194/acp-15-13665-2015
language
English
LU publication?
no
id
f8bebf1d-a527-45fe-9e12-a58b74583a8b
date added to LUP
2019-06-27 14:14:41
date last changed
2022-02-15 21:52:22
@article{f8bebf1d-a527-45fe-9e12-a58b74583a8b,
  abstract     = {{<p>Visible Multifilter Rotating Shadowband Radiometer (vis-MFRSR) data were collected at Storm Peak Laboratory (SPL), a mountain-top facility in northwest Colorado, from 1999 to 2011 and in 2013. From 2011 to 2014, in situ measurements of aerosol light scattering were also obtained. Using these data sets together, the seasonal impact of dust and biomass burning is considered for the western USA. Analysis indicates that the median contributions to spring and summer aerosol optical depth (AOD) from dust and biomass-burning aerosols across the data set are comparable. The mean AOD is slightly greater in the summer, with significantly more frequent and short-duration high AOD measurements due to biomass-burning episodes than in the spring. The Ångström exponent showed a significant increase in the summer for both the in situ and vis-MFRSR data, suggesting an increase in combustion aerosols. Spring dust events are less distinguishable in the in situ data than the column measurement, suggesting that a significant amount of dust may be found above the elevation of SPL, 3220 m a.s.l. Twenty-two known case studies of intercontinental dust, regional dust, and biomass-burning events were investigated. These events were found to follow a similar pattern, in both aerosol loading and Ångström exponent, as the seasonal mean signal in both the vis-MFRSR and ground-based nephelometer. This data set highlights the wide-scale implications of a warmer, drier climate on visibility in the western USA.</p>}},
  author       = {{Hallar, A. G. and Petersen, R. and Andrews, Elisabeth and Michalsky, J. and McCubbin, I. B. and Ogren, J. A.}},
  issn         = {{1680-7316}},
  language     = {{eng}},
  month        = {{12}},
  number       = {{23}},
  pages        = {{13665--13679}},
  publisher    = {{Copernicus GmbH}},
  series       = {{Atmospheric Chemistry and Physics}},
  title        = {{Contributions of dust and biomass burning to aerosols at a Colorado mountain-top site}},
  url          = {{http://dx.doi.org/10.5194/acp-15-13665-2015}},
  doi          = {{10.5194/acp-15-13665-2015}},
  volume       = {{15}},
  year         = {{2015}},
}