Nonperturbative modeling of fifth-order coherent multidimensional spectroscopy in light harvesting antennas
(2011) In New Journal of Physics 13(2).- Abstract
- Recent advances in coherent multidimensional spectroscopy have boosted interest in exciton coherences in light harvesting complexes. We present nonperturbative calculations of two-dimensional (2D) electronic spectroscopy from a fifth-order phase-matching direction. The calculations show clear patterns that correspond to the electronic structure of one- and two-exciton manifolds of a Fenna-Matthews-Olsson light harvesting complex. Such signals can provide new information about the coherent properties of antenna pigment protein complexes.
Please use this url to cite or link to this publication:
https://lup.lub.lu.se/record/1868948
- author
- Brueggemann, Ben and Pullerits, Tönu LU
- organization
- publishing date
- 2011
- type
- Contribution to journal
- publication status
- published
- subject
- in
- New Journal of Physics
- volume
- 13
- issue
- 2
- article number
- 025024
- publisher
- IOP Publishing
- external identifiers
-
- wos:000287857400001
- scopus:79952257004
- ISSN
- 1367-2630
- DOI
- 10.1088/1367-2630/13/2/025024
- language
- English
- LU publication?
- yes
- additional info
- The information about affiliations in this record was updated in December 2015. The record was previously connected to the following departments: Chemical Physics (S) (011001060)
- id
- f98c4e8e-52fd-4a86-92cf-a8a47d18f211 (old id 1868948)
- date added to LUP
- 2016-04-01 13:58:39
- date last changed
- 2023-09-03 07:49:07
@article{f98c4e8e-52fd-4a86-92cf-a8a47d18f211,
abstract = {{Recent advances in coherent multidimensional spectroscopy have boosted interest in exciton coherences in light harvesting complexes. We present nonperturbative calculations of two-dimensional (2D) electronic spectroscopy from a fifth-order phase-matching direction. The calculations show clear patterns that correspond to the electronic structure of one- and two-exciton manifolds of a Fenna-Matthews-Olsson light harvesting complex. Such signals can provide new information about the coherent properties of antenna pigment protein complexes.}},
author = {{Brueggemann, Ben and Pullerits, Tönu}},
issn = {{1367-2630}},
language = {{eng}},
number = {{2}},
publisher = {{IOP Publishing}},
series = {{New Journal of Physics}},
title = {{Nonperturbative modeling of fifth-order coherent multidimensional spectroscopy in light harvesting antennas}},
url = {{http://dx.doi.org/10.1088/1367-2630/13/2/025024}},
doi = {{10.1088/1367-2630/13/2/025024}},
volume = {{13}},
year = {{2011}},
}