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Large lattice distortions associated with the magnetic transition in La0.7Sr0.3MnO3

Weber, F. ; Argyriou, Dimitri LU ; Prokhnenko, O. and Reznik, D. (2013) In Physical Review B (Condensed Matter and Materials Physics) 88(24).
Abstract
Colossal magnetoresistance (CMR) is associated with the phase transition from a metallic ferromagnetic to insulating paramagnetic phase, which can be controlled by an applied magnetic field. The insulating phase occurs due to trapping of the charge carriers by polaronic lattice distortions, which raise the resistivity. Theories based on local physics predict that the magnitude of the resistivity jump at T-C is determined by how much, on average, the amplitude of these distortions increases at the phase transition. Using neutron scattering, we measured the average distortion amplitude in La0.7Sr0.3MnO3. Surprisingly, its increase from below to above T-C is just as large as in other manganites, which have a much larger resistivity jump. This... (More)
Colossal magnetoresistance (CMR) is associated with the phase transition from a metallic ferromagnetic to insulating paramagnetic phase, which can be controlled by an applied magnetic field. The insulating phase occurs due to trapping of the charge carriers by polaronic lattice distortions, which raise the resistivity. Theories based on local physics predict that the magnitude of the resistivity jump at T-C is determined by how much, on average, the amplitude of these distortions increases at the phase transition. Using neutron scattering, we measured the average distortion amplitude in La0.7Sr0.3MnO3. Surprisingly, its increase from below to above T-C is just as large as in other manganites, which have a much larger resistivity jump. This result suggests that the strength of CMR is determined not by the size of distortions, but by their cooperative nature, specific to each compound. Existing theories need to be extended to include correlations between different unit cells to explain and predict the strength of CMR. (Less)
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organization
publishing date
type
Contribution to journal
publication status
published
subject
in
Physical Review B (Condensed Matter and Materials Physics)
volume
88
issue
24
article number
241106
publisher
American Physical Society
external identifiers
  • wos:000328678600002
  • scopus:84890597130
ISSN
1098-0121
DOI
10.1103/PhysRevB.88.241106
language
English
LU publication?
yes
id
fc6ab973-e38b-41a0-a6d3-61af279229b1 (old id 4265889)
date added to LUP
2016-04-01 13:13:10
date last changed
2022-03-29 06:13:09
@article{fc6ab973-e38b-41a0-a6d3-61af279229b1,
  abstract     = {{Colossal magnetoresistance (CMR) is associated with the phase transition from a metallic ferromagnetic to insulating paramagnetic phase, which can be controlled by an applied magnetic field. The insulating phase occurs due to trapping of the charge carriers by polaronic lattice distortions, which raise the resistivity. Theories based on local physics predict that the magnitude of the resistivity jump at T-C is determined by how much, on average, the amplitude of these distortions increases at the phase transition. Using neutron scattering, we measured the average distortion amplitude in La0.7Sr0.3MnO3. Surprisingly, its increase from below to above T-C is just as large as in other manganites, which have a much larger resistivity jump. This result suggests that the strength of CMR is determined not by the size of distortions, but by their cooperative nature, specific to each compound. Existing theories need to be extended to include correlations between different unit cells to explain and predict the strength of CMR.}},
  author       = {{Weber, F. and Argyriou, Dimitri and Prokhnenko, O. and Reznik, D.}},
  issn         = {{1098-0121}},
  language     = {{eng}},
  number       = {{24}},
  publisher    = {{American Physical Society}},
  series       = {{Physical Review B (Condensed Matter and Materials Physics)}},
  title        = {{Large lattice distortions associated with the magnetic transition in La0.7Sr0.3MnO3}},
  url          = {{http://dx.doi.org/10.1103/PhysRevB.88.241106}},
  doi          = {{10.1103/PhysRevB.88.241106}},
  volume       = {{88}},
  year         = {{2013}},
}