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Evaluation of the in-situ performance of neutron detectors based on EJ-426 scintillator screens for spent fuel characterization

Perrey, Hanno LU ; Ros, Linus LU ; Elfman, Mikael LU ; Bäckström, Ulrika ; Kristiansson, Per LU and Sjöland, Anders LU (2021) In Nuclear Instruments and Methods in Physics Research, Section A: Accelerators, Spectrometers, Detectors and Associated Equipment 1020.
Abstract

The reliable detection of neutrons in a harsh gamma-ray environment is an important aspect of establishing non-destructive methods for the characterization of spent nuclear fuel. In this study, we present results from extended in-situ monitoring of detector systems consisting of commercially available components: EJ-426, a 6Li-enriched solid-state scintillator material sensitive to thermal neutrons, and two different types of Hamamatsu photomultiplier tubes (PMT). Over the period of eight months, these detectors were operated in close vicinity to spent nuclear fuel stored at the interim storage facility CLAB, Oskarshamn, Sweden. At the measurement position the detectors were continuously exposed to an estimated (moderated)... (More)

The reliable detection of neutrons in a harsh gamma-ray environment is an important aspect of establishing non-destructive methods for the characterization of spent nuclear fuel. In this study, we present results from extended in-situ monitoring of detector systems consisting of commercially available components: EJ-426, a 6Li-enriched solid-state scintillator material sensitive to thermal neutrons, and two different types of Hamamatsu photomultiplier tubes (PMT). Over the period of eight months, these detectors were operated in close vicinity to spent nuclear fuel stored at the interim storage facility CLAB, Oskarshamn, Sweden. At the measurement position the detectors were continuously exposed to an estimated (moderated) neutron flux of approx. 280n/scm2 and a gamma-ray dose rate of approximately 6Sv/h. Using offline software algorithms, neutron pulses were identified and characterized in the data. Over the entire investigated dose range of up to 35kGy, the detector systems were functioning and were delivering detectable neutron signals. Their performance as measured by the number of identified neutrons degrades down to about 30% of the initial value. Investigations of the irradiated components suggest that this degradation is a result of reduced optical transparency of the involved materials as well as a reduction of PMT gain due to the continuous high currents. Increasing the gain of the PMT through step-ups of the applied high voltage allowed to partially compensate for this loss in detection sensitivity even when the detectors were highly irradiated. The integrated neutron fluence during the measurement was experimentally verified to be in the order of 5×109ncm−2. The results were interpreted with the help of MCNP6.2 simulations of the setup and the neutron flux.

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author
; ; ; ; and
organization
publishing date
type
Contribution to journal
publication status
published
subject
keywords
EJ-426, Mixed-field radiation environment, Neutron detector, Photo-multiplier tube, Radiation hardness, Spent nuclear fuel characterization
in
Nuclear Instruments and Methods in Physics Research, Section A: Accelerators, Spectrometers, Detectors and Associated Equipment
volume
1020
article number
165886
publisher
Elsevier
external identifiers
  • scopus:85117785798
ISSN
0168-9002
DOI
10.1016/j.nima.2021.165886
language
English
LU publication?
yes
additional info
Publisher Copyright: © 2021 The Authors
id
0a863210-71f7-49eb-854d-966afdcdefcb
date added to LUP
2021-11-13 08:56:11
date last changed
2022-04-27 05:38:14
@article{0a863210-71f7-49eb-854d-966afdcdefcb,
  abstract     = {{<p>The reliable detection of neutrons in a harsh gamma-ray environment is an important aspect of establishing non-destructive methods for the characterization of spent nuclear fuel. In this study, we present results from extended in-situ monitoring of detector systems consisting of commercially available components: EJ-426, a <sup>6</sup>Li-enriched solid-state scintillator material sensitive to thermal neutrons, and two different types of Hamamatsu photomultiplier tubes (PMT). Over the period of eight months, these detectors were operated in close vicinity to spent nuclear fuel stored at the interim storage facility CLAB, Oskarshamn, Sweden. At the measurement position the detectors were continuously exposed to an estimated (moderated) neutron flux of approx. 280n/scm<sup>2</sup> and a gamma-ray dose rate of approximately 6Sv/h. Using offline software algorithms, neutron pulses were identified and characterized in the data. Over the entire investigated dose range of up to 35kGy, the detector systems were functioning and were delivering detectable neutron signals. Their performance as measured by the number of identified neutrons degrades down to about 30% of the initial value. Investigations of the irradiated components suggest that this degradation is a result of reduced optical transparency of the involved materials as well as a reduction of PMT gain due to the continuous high currents. Increasing the gain of the PMT through step-ups of the applied high voltage allowed to partially compensate for this loss in detection sensitivity even when the detectors were highly irradiated. The integrated neutron fluence during the measurement was experimentally verified to be in the order of 5×10<sup>9</sup>ncm<sup>−2</sup>. The results were interpreted with the help of MCNP6.2 simulations of the setup and the neutron flux.</p>}},
  author       = {{Perrey, Hanno and Ros, Linus and Elfman, Mikael and Bäckström, Ulrika and Kristiansson, Per and Sjöland, Anders}},
  issn         = {{0168-9002}},
  keywords     = {{EJ-426; Mixed-field radiation environment; Neutron detector; Photo-multiplier tube; Radiation hardness; Spent nuclear fuel characterization}},
  language     = {{eng}},
  month        = {{12}},
  publisher    = {{Elsevier}},
  series       = {{Nuclear Instruments and Methods in Physics Research, Section A: Accelerators, Spectrometers, Detectors and Associated Equipment}},
  title        = {{Evaluation of the in-situ performance of neutron detectors based on EJ-426 scintillator screens for spent fuel characterization}},
  url          = {{http://dx.doi.org/10.1016/j.nima.2021.165886}},
  doi          = {{10.1016/j.nima.2021.165886}},
  volume       = {{1020}},
  year         = {{2021}},
}