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Effect of bi-layer interconnector design on mass transfer performance in porous anode of solid oxide fuel cells

Chen, Qiuyang ; Wang, Qiuwang ; Zhang, Jian and Yuan, Jinliang LU (2011) In International Journal of Heat and Mass Transfer 54(9-10). p.1994-2003
Abstract
We propose a novel interconnector design, termed bi-layer interconnector, for solid oxide fuel cells (SOFCs). It can disturb the fuel gas and air on the planes normal to the SOFC three-phase-boundary (TPB) layer. In this paper, a two-dimensional half-cell model is developed to study the concentration overpotentials in the fuel side of the SOFC stack with conventional and novel bi-layer interconnectors. The numerical results show that the novel bi-layer interconnector can increase the velocity of the fuel gas in the porous anode. The results of mole fraction distribution illustrate that the novel bi-layer interconnector can effectively disturb the fuel flow. The average H-2 mole fraction in the porous anode of SOFC with bi-layer... (More)
We propose a novel interconnector design, termed bi-layer interconnector, for solid oxide fuel cells (SOFCs). It can disturb the fuel gas and air on the planes normal to the SOFC three-phase-boundary (TPB) layer. In this paper, a two-dimensional half-cell model is developed to study the concentration overpotentials in the fuel side of the SOFC stack with conventional and novel bi-layer interconnectors. The numerical results show that the novel bi-layer interconnector can increase the velocity of the fuel gas in the porous anode. The results of mole fraction distribution illustrate that the novel bi-layer interconnector can effectively disturb the fuel flow. The average H-2 mole fraction in the porous anode of SOFC with bi-layer interconnector is about 4.7% higher than that of conventional SOFC. The average H-2 mole fraction at TPB interface is about 9.2% higher. The concentration overpotential of the novel SOFC design is lower than that of the conventional SOFC design by 5%. It can enhance the mass transfer in porous electrode and improve the performance of SOFC. (C) 2011 Elsevier Ltd. All rights reserved. (Less)
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author
; ; and
organization
publishing date
type
Contribution to journal
publication status
published
subject
keywords
Solid oxide fuel cell, Bi-layer interconnector, Mass transfer, Concentration polarization, Half-cell model, Numerical simulation
in
International Journal of Heat and Mass Transfer
volume
54
issue
9-10
pages
1994 - 2003
publisher
Pergamon Press Ltd.
external identifiers
  • wos:000289011700030
  • scopus:79952282787
ISSN
0017-9310
DOI
10.1016/j.ijheatmasstransfer.2011.01.003
language
English
LU publication?
yes
id
c7911c3b-f4a4-4331-861b-81394d5338ed (old id 1925338)
date added to LUP
2016-04-01 10:26:45
date last changed
2022-04-27 22:08:35
@article{c7911c3b-f4a4-4331-861b-81394d5338ed,
  abstract     = {{We propose a novel interconnector design, termed bi-layer interconnector, for solid oxide fuel cells (SOFCs). It can disturb the fuel gas and air on the planes normal to the SOFC three-phase-boundary (TPB) layer. In this paper, a two-dimensional half-cell model is developed to study the concentration overpotentials in the fuel side of the SOFC stack with conventional and novel bi-layer interconnectors. The numerical results show that the novel bi-layer interconnector can increase the velocity of the fuel gas in the porous anode. The results of mole fraction distribution illustrate that the novel bi-layer interconnector can effectively disturb the fuel flow. The average H-2 mole fraction in the porous anode of SOFC with bi-layer interconnector is about 4.7% higher than that of conventional SOFC. The average H-2 mole fraction at TPB interface is about 9.2% higher. The concentration overpotential of the novel SOFC design is lower than that of the conventional SOFC design by 5%. It can enhance the mass transfer in porous electrode and improve the performance of SOFC. (C) 2011 Elsevier Ltd. All rights reserved.}},
  author       = {{Chen, Qiuyang and Wang, Qiuwang and Zhang, Jian and Yuan, Jinliang}},
  issn         = {{0017-9310}},
  keywords     = {{Solid oxide fuel cell; Bi-layer interconnector; Mass transfer; Concentration polarization; Half-cell model; Numerical simulation}},
  language     = {{eng}},
  number       = {{9-10}},
  pages        = {{1994--2003}},
  publisher    = {{Pergamon Press Ltd.}},
  series       = {{International Journal of Heat and Mass Transfer}},
  title        = {{Effect of bi-layer interconnector design on mass transfer performance in porous anode of solid oxide fuel cells}},
  url          = {{http://dx.doi.org/10.1016/j.ijheatmasstransfer.2011.01.003}},
  doi          = {{10.1016/j.ijheatmasstransfer.2011.01.003}},
  volume       = {{54}},
  year         = {{2011}},
}