Spatial quantum beats in vibrational resonant inelastic soft x-ray scattering at dissociating States in oxygen.
(2011) In Physical Review Letters 106(15).- Abstract
- Resonant inelastic soft x-ray scattering (RIXS) spectra excited at the 1σ_{g}→3σ_{u} resonance in gas-phase O_{2} show excitations due to the nuclear degrees of freedom with up to 35 well-resolved discrete vibronic states and a continuum due to the kinetic energy distribution of the separated atoms. The RIXS profile demonstrates spatial quantum beats caused by two interfering wave packets with different momenta as the atoms separate. Thomson scattering strongly affects both the spectral profile and the scattering anisotropy.
Please use this url to cite or link to this publication:
https://lup.lub.lu.se/record/1972639
- author
- organization
- publishing date
- 2011
- type
- Contribution to journal
- publication status
- published
- subject
- in
- Physical Review Letters
- volume
- 106
- issue
- 15
- article number
- 153004
- publisher
- American Physical Society
- external identifiers
-
- wos:000289525300005
- pmid:21568552
- scopus:79960623604
- pmid:21568552
- ISSN
- 1079-7114
- DOI
- 10.1103/PhysRevLett.106.153004
- language
- English
- LU publication?
- yes
- id
- c20646eb-7b68-4122-9cc2-6a41c76f35a5 (old id 1972639)
- date added to LUP
- 2016-04-01 10:36:19
- date last changed
- 2022-04-04 19:37:29
@article{c20646eb-7b68-4122-9cc2-6a41c76f35a5, abstract = {{Resonant inelastic soft x-ray scattering (RIXS) spectra excited at the 1σ_{g}→3σ_{u} resonance in gas-phase O_{2} show excitations due to the nuclear degrees of freedom with up to 35 well-resolved discrete vibronic states and a continuum due to the kinetic energy distribution of the separated atoms. The RIXS profile demonstrates spatial quantum beats caused by two interfering wave packets with different momenta as the atoms separate. Thomson scattering strongly affects both the spectral profile and the scattering anisotropy.}}, author = {{Pietzsch, Annette and Sun, Y and Hennies, Franz and Rinkevicius, Z and Karlsson, H O and Schmitt, T and Strocov, V N and Andersson, J and Kennedy, B and Schlappa, J and Föhlisch, A and Rubensson, J-E and Gel'mukhanov, F}}, issn = {{1079-7114}}, language = {{eng}}, number = {{15}}, publisher = {{American Physical Society}}, series = {{Physical Review Letters}}, title = {{Spatial quantum beats in vibrational resonant inelastic soft x-ray scattering at dissociating States in oxygen.}}, url = {{http://dx.doi.org/10.1103/PhysRevLett.106.153004}}, doi = {{10.1103/PhysRevLett.106.153004}}, volume = {{106}}, year = {{2011}}, }