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Extended X-ray absorption spectroscopy using an ultrashort pulse laboratory-scale laser-plasma accelerator

Kettle, Brendan ; Colgan, Cary ; Los, Eva E. ; Gerstmayr, Elias ; Streeter, Matthew J.V. ; Albert, Felicie ; Astbury, Sam ; Baggott, Rory A. ; Cavanagh, Niall and Falk, Kateřina , et al. (2024) In Communications Physics 7(1).
Abstract

Laser-driven compact particle accelerators can provide ultrashort pulses of broadband X-rays, well suited for undertaking X-ray absorption spectroscopy measurements on a femtosecond timescale. Here the Extended X-ray Absorption Fine Structure (EXAFS) features of the K-edge of a copper sample have been observed over a 250 eV window in a single shot using a laser wakefield accelerator, providing information on both the electronic and ionic structure simultaneously. This capability will allow the investigation of ultrafast processes, and in particular, probing high-energy-density matter and physics far-from-equilibrium where the sample refresh rate is slow and shot number is limited. For example, states that replicate the tremendous... (More)

Laser-driven compact particle accelerators can provide ultrashort pulses of broadband X-rays, well suited for undertaking X-ray absorption spectroscopy measurements on a femtosecond timescale. Here the Extended X-ray Absorption Fine Structure (EXAFS) features of the K-edge of a copper sample have been observed over a 250 eV window in a single shot using a laser wakefield accelerator, providing information on both the electronic and ionic structure simultaneously. This capability will allow the investigation of ultrafast processes, and in particular, probing high-energy-density matter and physics far-from-equilibrium where the sample refresh rate is slow and shot number is limited. For example, states that replicate the tremendous pressures and temperatures of planetary bodies or the conditions inside nuclear fusion reactions. Using high-power lasers to pump these samples also has the advantage of being inherently synchronised to the laser-driven X-ray probe. A perspective on the additional strengths of a laboratory-based ultrafast X-ray absorption source is presented.

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Please use this url to cite or link to this publication:
@article{58af2e8b-287e-49c7-9491-86e0af7c713a,
  abstract     = {{<p>Laser-driven compact particle accelerators can provide ultrashort pulses of broadband X-rays, well suited for undertaking X-ray absorption spectroscopy measurements on a femtosecond timescale. Here the Extended X-ray Absorption Fine Structure (EXAFS) features of the K-edge of a copper sample have been observed over a 250 eV window in a single shot using a laser wakefield accelerator, providing information on both the electronic and ionic structure simultaneously. This capability will allow the investigation of ultrafast processes, and in particular, probing high-energy-density matter and physics far-from-equilibrium where the sample refresh rate is slow and shot number is limited. For example, states that replicate the tremendous pressures and temperatures of planetary bodies or the conditions inside nuclear fusion reactions. Using high-power lasers to pump these samples also has the advantage of being inherently synchronised to the laser-driven X-ray probe. A perspective on the additional strengths of a laboratory-based ultrafast X-ray absorption source is presented.</p>}},
  author       = {{Kettle, Brendan and Colgan, Cary and Los, Eva E. and Gerstmayr, Elias and Streeter, Matthew J.V. and Albert, Felicie and Astbury, Sam and Baggott, Rory A. and Cavanagh, Niall and Falk, Kateřina and Hyde, Timothy I. and Lundh, Olle and Rajeev, P. Pattathil and Riley, Dave and Rose, Steven J. and Sarri, Gianluca and Spindloe, Chris and Svendsen, Kristoffer and Symes, Dan R. and Šmíd, Michal and Thomas, Alec G.R. and Thornton, Chris and Watt, Robbie and Mangles, Stuart P.D.}},
  issn         = {{2399-3650}},
  language     = {{eng}},
  number       = {{1}},
  publisher    = {{Nature Publishing Group}},
  series       = {{Communications Physics}},
  title        = {{Extended X-ray absorption spectroscopy using an ultrashort pulse laboratory-scale laser-plasma accelerator}},
  url          = {{http://dx.doi.org/10.1038/s42005-024-01735-1}},
  doi          = {{10.1038/s42005-024-01735-1}},
  volume       = {{7}},
  year         = {{2024}},
}