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Comment on "review of experimental studies of secondary ice production" by Korolev and Leisner (2020)

Phillips, Vaughan T.J. LU orcid ; Yano, Jun Ichi ; Deshmukh, Akash LU and Waman, Deepak LU orcid (2021) In Atmospheric Chemistry and Physics 21(15). p.11941-11953
Abstract

This is a comment on the review by Korolev and Leisner (2020, hereafter KL2020). The only two laboratory/field studies ever to measure the breakup in ice-ice collisions for in-cloud conditions were negatively criticised by KL2020, as were our subsequent theoretical and modelling studies informed by both studies. First, hypothetically, even without any further laboratory experiments, such theoretical and modelling studies would continue to be possible, based on classical mechanics and statistical physics. They are not sensitive to the accuracy of lab data for typical situations, partly because the nonlinear explosive growth of ice concentrations continues until some maximum concentration is reached. To a degree, the same final... (More)

This is a comment on the review by Korolev and Leisner (2020, hereafter KL2020). The only two laboratory/field studies ever to measure the breakup in ice-ice collisions for in-cloud conditions were negatively criticised by KL2020, as were our subsequent theoretical and modelling studies informed by both studies. First, hypothetically, even without any further laboratory experiments, such theoretical and modelling studies would continue to be possible, based on classical mechanics and statistical physics. They are not sensitive to the accuracy of lab data for typical situations, partly because the nonlinear explosive growth of ice concentrations continues until some maximum concentration is reached. To a degree, the same final concentration is expected regardless of the fragment number per collision. Second, there is no evidence that both lab/field observational studies characterising fragmentation in ice-ice collisions are either mutually conflicting or erroneous such that they cannot be used to represent this breakup in numerical models, contrary to the review. The fact that the ice spheres of one experiment were hail sized (2ĝ€¯cm) is not a problem if a universal theoretical formulation, such as ours, with fundamental dependencies, is informed by it. Although both lab/field studies involved head-on collisions, rotational kinetic energy for all collisions generally is only a small fraction of the initial collision kinetic energy (CKE) anyway. Although both lab/field experiments involved fixed targets, that is not a problem since the fixing of the target is represented via CKE in any energy-based formulation such as ours. Finally, scaling analysis suggests that the breakup of ice during sublimation can make a significant contribution to ice enhancement in clouds, again contrary to the impression given by the review.

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author
; ; and
organization
publishing date
type
Contribution to journal
publication status
published
subject
in
Atmospheric Chemistry and Physics
volume
21
issue
15
pages
13 pages
publisher
Copernicus GmbH
external identifiers
  • scopus:85113170876
ISSN
1680-7316
DOI
10.5194/acp-21-11941-2021
project
Secondary ice production: An empirical formulation and organization of mechanisms among simulated cloud-types
language
English
LU publication?
yes
id
c04d8bb3-dfb0-4ad6-a508-f9a4b049e7e4
date added to LUP
2021-09-07 13:44:32
date last changed
2023-10-25 07:24:33
@article{c04d8bb3-dfb0-4ad6-a508-f9a4b049e7e4,
  abstract     = {{<p>This is a comment on the review by Korolev and Leisner (2020, hereafter KL2020). The only two laboratory/field studies ever to measure the breakup in ice-ice collisions for in-cloud conditions were negatively criticised by KL2020, as were our subsequent theoretical and modelling studies informed by both studies. First, hypothetically, even without any further laboratory experiments, such theoretical and modelling studies would continue to be possible, based on classical mechanics and statistical physics. They are not sensitive to the accuracy of lab data for typical situations, partly because the nonlinear explosive growth of ice concentrations continues until some maximum concentration is reached. To a degree, the same final concentration is expected regardless of the fragment number per collision. Second, there is no evidence that both lab/field observational studies characterising fragmentation in ice-ice collisions are either mutually conflicting or erroneous such that they cannot be used to represent this breakup in numerical models, contrary to the review. The fact that the ice spheres of one experiment were hail sized (2ĝ€¯cm) is not a problem if a universal theoretical formulation, such as ours, with fundamental dependencies, is informed by it. Although both lab/field studies involved head-on collisions, rotational kinetic energy for all collisions generally is only a small fraction of the initial collision kinetic energy (CKE) anyway. Although both lab/field experiments involved fixed targets, that is not a problem since the fixing of the target is represented via CKE in any energy-based formulation such as ours. Finally, scaling analysis suggests that the breakup of ice during sublimation can make a significant contribution to ice enhancement in clouds, again contrary to the impression given by the review. </p>}},
  author       = {{Phillips, Vaughan T.J. and Yano, Jun Ichi and Deshmukh, Akash and Waman, Deepak}},
  issn         = {{1680-7316}},
  language     = {{eng}},
  number       = {{15}},
  pages        = {{11941--11953}},
  publisher    = {{Copernicus GmbH}},
  series       = {{Atmospheric Chemistry and Physics}},
  title        = {{Comment on "review of experimental studies of secondary ice production" by Korolev and Leisner (2020)}},
  url          = {{http://dx.doi.org/10.5194/acp-21-11941-2021}},
  doi          = {{10.5194/acp-21-11941-2021}},
  volume       = {{21}},
  year         = {{2021}},
}