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Gaining control on optical force by the stimulated-emission resonance effect

Kudo, Tetsuhiro ; Louis, Boris LU ; Sotome, Hikaru ; Chen, Jui Kai ; Ito, Syoji ; Miyasaka, Hiroshi ; Masuhara, Hiroshi ; Hofkens, Johan and Bresolí-Obach, Roger (2023) In Chemical Science 14(37). p.10087-10095
Abstract

The resonance between an electronic transition of a micro/nanoscale object and an incident photon flux can modify the radiation force exerted on that object, especially at an interface. It has been theoretically proposed that a non-linear stimulated emission process can also induce an optical force, however its direction will be opposite to conventional photon scattering/absorption processes. In this work, we experimentally and theoretically demonstrate that a stimulated emission process can induce a repulsive pulling optical force on a single trapped dye-doped particle. Moreover, we successfully integrate both attractive pushing (excited state absorption) and repulsive pulling (stimulated emission) resonance forces to control the... (More)

The resonance between an electronic transition of a micro/nanoscale object and an incident photon flux can modify the radiation force exerted on that object, especially at an interface. It has been theoretically proposed that a non-linear stimulated emission process can also induce an optical force, however its direction will be opposite to conventional photon scattering/absorption processes. In this work, we experimentally and theoretically demonstrate that a stimulated emission process can induce a repulsive pulling optical force on a single trapped dye-doped particle. Moreover, we successfully integrate both attractive pushing (excited state absorption) and repulsive pulling (stimulated emission) resonance forces to control the overall exerted optical force on an object, validating the proposed non-linear optical resonance theory. Indeed, the results presented here will enable the optical manipulation of the exerted optical force with exquisite control and ultimately enable single particle manipulation.

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author
; ; ; ; ; ; ; and
organization
publishing date
type
Contribution to journal
publication status
published
subject
in
Chemical Science
volume
14
issue
37
pages
9 pages
publisher
Royal Society of Chemistry
external identifiers
  • pmid:37772121
  • scopus:85170249012
ISSN
2041-6520
DOI
10.1039/d3sc01927f
language
English
LU publication?
yes
id
0a2e5be8-a153-475f-9ad9-996c4a367271
date added to LUP
2023-12-22 09:29:09
date last changed
2024-04-20 18:49:36
@article{0a2e5be8-a153-475f-9ad9-996c4a367271,
  abstract     = {{<p>The resonance between an electronic transition of a micro/nanoscale object and an incident photon flux can modify the radiation force exerted on that object, especially at an interface. It has been theoretically proposed that a non-linear stimulated emission process can also induce an optical force, however its direction will be opposite to conventional photon scattering/absorption processes. In this work, we experimentally and theoretically demonstrate that a stimulated emission process can induce a repulsive pulling optical force on a single trapped dye-doped particle. Moreover, we successfully integrate both attractive pushing (excited state absorption) and repulsive pulling (stimulated emission) resonance forces to control the overall exerted optical force on an object, validating the proposed non-linear optical resonance theory. Indeed, the results presented here will enable the optical manipulation of the exerted optical force with exquisite control and ultimately enable single particle manipulation.</p>}},
  author       = {{Kudo, Tetsuhiro and Louis, Boris and Sotome, Hikaru and Chen, Jui Kai and Ito, Syoji and Miyasaka, Hiroshi and Masuhara, Hiroshi and Hofkens, Johan and Bresolí-Obach, Roger}},
  issn         = {{2041-6520}},
  language     = {{eng}},
  month        = {{08}},
  number       = {{37}},
  pages        = {{10087--10095}},
  publisher    = {{Royal Society of Chemistry}},
  series       = {{Chemical Science}},
  title        = {{Gaining control on optical force by the stimulated-emission resonance effect}},
  url          = {{http://dx.doi.org/10.1039/d3sc01927f}},
  doi          = {{10.1039/d3sc01927f}},
  volume       = {{14}},
  year         = {{2023}},
}