Nature of Metallic and Insulating Domains in the Charge-Density-Wave System 1T-TaSe_{2}
(2025) In Physical Review Letters 135(9). p.96501-96501- Abstract
We study the electronic structure of bulk 1T-TaSe_{2} in the charge-density wave phase at low temperature. Our spatially and angle-resolved photoemission data show insulating areas coexisting with metallic regions characterized by a chiral Fermi surface and moderately correlated quasiparticle bands. Additionally, high-resolution laser angle-resolved photoemission reveals variations in the metallic regions, with series of low-energy states, whose energy, number, and dispersion can be explained by the formation of quantum well states of different thicknesses. Dynamical mean field theory calculations show that the observed rich behavior can be rationalized by assuming occasional stacking faults of the charge density wave. Our results... (More)
We study the electronic structure of bulk 1T-TaSe_{2} in the charge-density wave phase at low temperature. Our spatially and angle-resolved photoemission data show insulating areas coexisting with metallic regions characterized by a chiral Fermi surface and moderately correlated quasiparticle bands. Additionally, high-resolution laser angle-resolved photoemission reveals variations in the metallic regions, with series of low-energy states, whose energy, number, and dispersion can be explained by the formation of quantum well states of different thicknesses. Dynamical mean field theory calculations show that the observed rich behavior can be rationalized by assuming occasional stacking faults of the charge density wave. Our results indicate that the diverse electronic phenomena reported previously in 1T-TaSe_{2} are dictated by the stacking arrangement and the resulting quantum size effects while correlation effects play a secondary role.
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- author
- organization
- publishing date
- 2025-08
- type
- Contribution to journal
- publication status
- published
- subject
- in
- Physical Review Letters
- volume
- 135
- issue
- 9
- pages
- 1 pages
- publisher
- American Physical Society
- external identifiers
-
- scopus:105016275059
- pmid:40952233
- ISSN
- 1079-7114
- DOI
- 10.1103/pbyw-mzfy
- language
- English
- LU publication?
- yes
- id
- 0f9c464c-2602-494a-ab02-36b94082cf4b
- date added to LUP
- 2025-10-20 13:27:10
- date last changed
- 2025-11-17 15:29:52
@article{0f9c464c-2602-494a-ab02-36b94082cf4b,
abstract = {{<p>We study the electronic structure of bulk 1T-TaSe_{2} in the charge-density wave phase at low temperature. Our spatially and angle-resolved photoemission data show insulating areas coexisting with metallic regions characterized by a chiral Fermi surface and moderately correlated quasiparticle bands. Additionally, high-resolution laser angle-resolved photoemission reveals variations in the metallic regions, with series of low-energy states, whose energy, number, and dispersion can be explained by the formation of quantum well states of different thicknesses. Dynamical mean field theory calculations show that the observed rich behavior can be rationalized by assuming occasional stacking faults of the charge density wave. Our results indicate that the diverse electronic phenomena reported previously in 1T-TaSe_{2} are dictated by the stacking arrangement and the resulting quantum size effects while correlation effects play a secondary role.</p>}},
author = {{Straub, M. and Petocchi, F. and Witteveen, C. and Kugler, F. B. and Hunter, A. and Alexanian, Y. and Gatti, G. and Mandloi, S. and Polley, C. and Carbone, G. and Osiecki, J. and von Rohr, F. O. and Georges, A. and Baumberger, F. and Tamai, A.}},
issn = {{1079-7114}},
language = {{eng}},
number = {{9}},
pages = {{96501--96501}},
publisher = {{American Physical Society}},
series = {{Physical Review Letters}},
title = {{Nature of Metallic and Insulating Domains in the Charge-Density-Wave System 1T-TaSe_{2}}},
url = {{http://dx.doi.org/10.1103/pbyw-mzfy}},
doi = {{10.1103/pbyw-mzfy}},
volume = {{135}},
year = {{2025}},
}