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Droplet thermometry based on an optimized two dye two-color laser-induced fluorescence concept

Ulrich, Hannah ; Sigl, Sophie ; Möhnle, Michael ; Berrocal, Edouard LU and Zigan, Lars (2023) In Frontiers in Physics 11.
Abstract

In this work two-color laser-induced fluorescence (2c-LIF) is applied to calibrate and measure the temperature in a micrometric monodisperse ethanol droplet chain. A dye mixture of fluorescein disodium (FL) and sulforhodamine 101 (SRh) is used, in order to form a sensitive signal ratio of one temperature dependent and one independent fluorophore. Spectral and planar fluorescence detection via a fiber-coupled spectrometer and a camera system, consisting of two sCMOS cameras, is set up around the droplet chain. Additionally, absorption measurements of the dye mixture in ethanol are conducted using a photo-spectrometer to analyze the temperature sensitivity of the dyes as well as potential re-absorption and fluorescence cross-talk effects.... (More)

In this work two-color laser-induced fluorescence (2c-LIF) is applied to calibrate and measure the temperature in a micrometric monodisperse ethanol droplet chain. A dye mixture of fluorescein disodium (FL) and sulforhodamine 101 (SRh) is used, in order to form a sensitive signal ratio of one temperature dependent and one independent fluorophore. Spectral and planar fluorescence detection via a fiber-coupled spectrometer and a camera system, consisting of two sCMOS cameras, is set up around the droplet chain. Additionally, absorption measurements of the dye mixture in ethanol are conducted using a photo-spectrometer to analyze the temperature sensitivity of the dyes as well as potential re-absorption and fluorescence cross-talk effects. The spectral setup allowed an investigation of the wavelength range in which morphology dependent resonances (MDR) occur at the phase boundary of the droplet. Thus, the optical filters, determining the color channels in the camera system, are chosen to avoid detection of the lasing signal and providing maximal temperature sensitivity at the same time. The calibrated signal ratios are applied in temperature measurements of evaporating heated droplets in the droplet chain, showing the cooling with larger distance from the nozzle.

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author
; ; ; and
organization
publishing date
type
Contribution to journal
publication status
published
subject
keywords
2c-LIF, droplet cooling, droplets, dye, evaporation, fluorescence, thermometry
in
Frontiers in Physics
volume
11
article number
1235847
publisher
Frontiers Media S. A.
external identifiers
  • scopus:85168242796
ISSN
2296-424X
DOI
10.3389/fphy.2023.1235847
language
English
LU publication?
yes
id
0fcbad6a-9092-4e2c-9ad7-ff1c637506b4
date added to LUP
2023-12-22 17:05:38
date last changed
2023-12-22 17:06:16
@article{0fcbad6a-9092-4e2c-9ad7-ff1c637506b4,
  abstract     = {{<p>In this work two-color laser-induced fluorescence (2c-LIF) is applied to calibrate and measure the temperature in a micrometric monodisperse ethanol droplet chain. A dye mixture of fluorescein disodium (FL) and sulforhodamine 101 (SRh) is used, in order to form a sensitive signal ratio of one temperature dependent and one independent fluorophore. Spectral and planar fluorescence detection via a fiber-coupled spectrometer and a camera system, consisting of two sCMOS cameras, is set up around the droplet chain. Additionally, absorption measurements of the dye mixture in ethanol are conducted using a photo-spectrometer to analyze the temperature sensitivity of the dyes as well as potential re-absorption and fluorescence cross-talk effects. The spectral setup allowed an investigation of the wavelength range in which morphology dependent resonances (MDR) occur at the phase boundary of the droplet. Thus, the optical filters, determining the color channels in the camera system, are chosen to avoid detection of the lasing signal and providing maximal temperature sensitivity at the same time. The calibrated signal ratios are applied in temperature measurements of evaporating heated droplets in the droplet chain, showing the cooling with larger distance from the nozzle.</p>}},
  author       = {{Ulrich, Hannah and Sigl, Sophie and Möhnle, Michael and Berrocal, Edouard and Zigan, Lars}},
  issn         = {{2296-424X}},
  keywords     = {{2c-LIF; droplet cooling; droplets; dye; evaporation; fluorescence; thermometry}},
  language     = {{eng}},
  publisher    = {{Frontiers Media S. A.}},
  series       = {{Frontiers in Physics}},
  title        = {{Droplet thermometry based on an optimized two dye two-color laser-induced fluorescence concept}},
  url          = {{http://dx.doi.org/10.3389/fphy.2023.1235847}},
  doi          = {{10.3389/fphy.2023.1235847}},
  volume       = {{11}},
  year         = {{2023}},
}