Closed-loop upcycling of sewage sludge products into sp2-C-rich electrodes for pollutant oxidation : tracking mineralization by 14C-labeling
(2025) In Chemical Engineering Journal 520.- Abstract
To address the need for sustainable wastewater treatment, we developed sp2‑carbon-rich, hierarchically porous electrodes by upcycling sewage sludge ash (SSA) and biochar (CB) using a hybrid 3D printing and microwave plasma-enhanced chemical vapor deposition (MPECVD) approach. The CB-containing electrode exhibited a 260-fold increase in BET surface area (0.15 to 40.6 m2 g−1), but the lowest electrochemically active surface area (EASA = 18.3 cm2 g−1), indicating limited site accessibility. In contrast, SSA-based electrodes offered both higher BET and EASA values (up to 328.6 cm2 g−1), improving adsorption and oxidation performance. Electrochemical oxidation of... (More)
To address the need for sustainable wastewater treatment, we developed sp2‑carbon-rich, hierarchically porous electrodes by upcycling sewage sludge ash (SSA) and biochar (CB) using a hybrid 3D printing and microwave plasma-enhanced chemical vapor deposition (MPECVD) approach. The CB-containing electrode exhibited a 260-fold increase in BET surface area (0.15 to 40.6 m2 g−1), but the lowest electrochemically active surface area (EASA = 18.3 cm2 g−1), indicating limited site accessibility. In contrast, SSA-based electrodes offered both higher BET and EASA values (up to 328.6 cm2 g−1), improving adsorption and oxidation performance. Electrochemical oxidation of 14C-labelled micropollutants (BPA, diclofenac, carbamazepine, and PFOA) exhibited pollutant-specific removal pathways. SSA electrodes enhanced BPA adsorption and mineralization, achieving a 1.6-fold faster 14CO₂ production rate. While CBZ and DIC were partially mineralised, no measurable 14CO₂ formation was observed for PFOA, suggesting a different removal mechanism. An inverse correlation was observed between mineralization rates and DFT-calculated bond cleavage energies. These findings highlight the practical potential of upcycled electrodes to achieve efficient mineralization of persistent organic pollutants. This closed-loop strategy offers an environmentally viable approach to turning waste into functional materials for advanced wastewater treatment processes.
(Less)
- author
- Łepek, Angelika
; Szopińska, Małgorzata
; Kaczmarzyk, Iwona
; Olejnik, Adrian
; Falås, Per
LU
; Davidsson, Åsa
LU
; Cimbritz, Michael LU ; Gamoń, Filip and Pierpaoli, Mattia LU
- organization
- publishing date
- 2025-09-15
- type
- Contribution to journal
- publication status
- published
- subject
- keywords
- Carbon-based electrodes, DFT simulations, Electrochemical oxidation, Persistent organic pollutants, Upcycling, Wastewater treatment
- in
- Chemical Engineering Journal
- volume
- 520
- article number
- 166284
- pages
- 10 pages
- publisher
- Elsevier
- external identifiers
-
- scopus:105011478804
- ISSN
- 1385-8947
- DOI
- 10.1016/j.cej.2025.166284
- language
- English
- LU publication?
- yes
- additional info
- Publisher Copyright: © 2025 The Author(s)
- id
- 1c5c89a4-38c2-433e-9360-f5f833fc8214
- date added to LUP
- 2025-08-25 11:07:45
- date last changed
- 2025-08-25 13:53:35
@article{1c5c89a4-38c2-433e-9360-f5f833fc8214, abstract = {{<p>To address the need for sustainable wastewater treatment, we developed sp<sup>2</sup>‑carbon-rich, hierarchically porous electrodes by upcycling sewage sludge ash (SSA) and biochar (CB) using a hybrid 3D printing and microwave plasma-enhanced chemical vapor deposition (MPECVD) approach. The CB-containing electrode exhibited a 260-fold increase in BET surface area (0.15 to 40.6 m<sup>2</sup> g<sup>−1</sup>), but the lowest electrochemically active surface area (EASA = 18.3 cm<sup>2</sup> g<sup>−1</sup>), indicating limited site accessibility. In contrast, SSA-based electrodes offered both higher BET and EASA values (up to 328.6 cm<sup>2</sup> g<sup>−1</sup>), improving adsorption and oxidation performance. Electrochemical oxidation of <sup>14</sup>C-labelled micropollutants (BPA, diclofenac, carbamazepine, and PFOA) exhibited pollutant-specific removal pathways. SSA electrodes enhanced BPA adsorption and mineralization, achieving a 1.6-fold faster <sup>14</sup>CO₂ production rate. While CBZ and DIC were partially mineralised, no measurable <sup>14</sup>CO₂ formation was observed for PFOA, suggesting a different removal mechanism. An inverse correlation was observed between mineralization rates and DFT-calculated bond cleavage energies. These findings highlight the practical potential of upcycled electrodes to achieve efficient mineralization of persistent organic pollutants. This closed-loop strategy offers an environmentally viable approach to turning waste into functional materials for advanced wastewater treatment processes.</p>}}, author = {{Łepek, Angelika and Szopińska, Małgorzata and Kaczmarzyk, Iwona and Olejnik, Adrian and Falås, Per and Davidsson, Åsa and Cimbritz, Michael and Gamoń, Filip and Pierpaoli, Mattia}}, issn = {{1385-8947}}, keywords = {{Carbon-based electrodes; DFT simulations; Electrochemical oxidation; Persistent organic pollutants; Upcycling; Wastewater treatment}}, language = {{eng}}, month = {{09}}, publisher = {{Elsevier}}, series = {{Chemical Engineering Journal}}, title = {{Closed-loop upcycling of sewage sludge products into sp<sup>2</sup>-C-rich electrodes for pollutant oxidation : tracking mineralization by <sup>14</sup>C-labeling}}, url = {{http://dx.doi.org/10.1016/j.cej.2025.166284}}, doi = {{10.1016/j.cej.2025.166284}}, volume = {{520}}, year = {{2025}}, }