One-dimensional arrays of nanoshell dimers for single molecule spectroscopy via surface-enhanced raman scattering
(2006) In Journal of Chemical Physics 125(8).- Abstract
- The optical properties of one-dimensional arrays of metal nanoshell dimers are studied systematically using the T-matrix method based on Mie theory, within the context of surface enhanced Raman scattering (SERS). It is shown that the local electromagnetic enhancement can be as high as similar to 4.5x10(13) for nanoshell dimer arrays with optimal geometry, and sensitive tunability in the resonant frequency can be gained by varying the geometrical parameters, making such structures appealing templates for SERS measurements with single molecule sensitivity. The extraordinarily high enhancement is attributed to a collective photonic effect constructively superposed onto the intrinsic enhancement associated with an isolated nanoshell dimer. (c)... (More)
- The optical properties of one-dimensional arrays of metal nanoshell dimers are studied systematically using the T-matrix method based on Mie theory, within the context of surface enhanced Raman scattering (SERS). It is shown that the local electromagnetic enhancement can be as high as similar to 4.5x10(13) for nanoshell dimer arrays with optimal geometry, and sensitive tunability in the resonant frequency can be gained by varying the geometrical parameters, making such structures appealing templates for SERS measurements with single molecule sensitivity. The extraordinarily high enhancement is attributed to a collective photonic effect constructively superposed onto the intrinsic enhancement associated with an isolated nanoshell dimer. (c) 2006 American Institute of Physics. (Less)
Please use this url to cite or link to this publication:
https://lup.lub.lu.se/record/394737
- author
- Zhao, Ke ; Xu, Hongxing LU ; Gu, Baohua and Zhang, Zhenyu
- organization
- publishing date
- 2006
- type
- Contribution to journal
- publication status
- published
- subject
- in
- Journal of Chemical Physics
- volume
- 125
- issue
- 8
- article number
- 081102
- publisher
- American Institute of Physics (AIP)
- external identifiers
-
- wos:000240237000002
- scopus:33748260573
- pmid:16964992
- ISSN
- 0021-9606
- DOI
- 10.1063/1.2229204
- language
- English
- LU publication?
- yes
- id
- 0f91dc35-5013-4ef4-b081-120d1f39bd56 (old id 394737)
- date added to LUP
- 2016-04-01 12:33:06
- date last changed
- 2022-02-26 08:38:36
@article{0f91dc35-5013-4ef4-b081-120d1f39bd56, abstract = {{The optical properties of one-dimensional arrays of metal nanoshell dimers are studied systematically using the T-matrix method based on Mie theory, within the context of surface enhanced Raman scattering (SERS). It is shown that the local electromagnetic enhancement can be as high as similar to 4.5x10(13) for nanoshell dimer arrays with optimal geometry, and sensitive tunability in the resonant frequency can be gained by varying the geometrical parameters, making such structures appealing templates for SERS measurements with single molecule sensitivity. The extraordinarily high enhancement is attributed to a collective photonic effect constructively superposed onto the intrinsic enhancement associated with an isolated nanoshell dimer. (c) 2006 American Institute of Physics.}}, author = {{Zhao, Ke and Xu, Hongxing and Gu, Baohua and Zhang, Zhenyu}}, issn = {{0021-9606}}, language = {{eng}}, number = {{8}}, publisher = {{American Institute of Physics (AIP)}}, series = {{Journal of Chemical Physics}}, title = {{One-dimensional arrays of nanoshell dimers for single molecule spectroscopy via surface-enhanced raman scattering}}, url = {{http://dx.doi.org/10.1063/1.2229204}}, doi = {{10.1063/1.2229204}}, volume = {{125}}, year = {{2006}}, }