Intramolecular vibronic dynamics in molecular solids: C60
Kjeldgaard, Lisbeth LU ; Käämbre, Tanel LU ; Schiessling, Joachim ; Marenne, Ingrid ; O'Shea, James N. ; Schnadt, Joachim LU
; Glover, Chris J.
; Nagasono, Mitsuru
; Nordlund, Dennis
and Garnier, M. Gunnar
, et al.
(2005)
In Physical Review B (Condensed Matter and Materials Physics)
72(20).
- Abstract
- Vibronic coupling in solid C60 has been investigated with a combination of resonant photoemission spectroscopy (RPES) and resonant inelastic x-ray scattering (RIXS). Excitation as a function of energy within the lowest unoccupied molecular orbital resonance yielded strong oscillations in intensity and dispersion in RPES, and a strong inelastic component in RIXS. Reconciling these two observations establishes that vibronic coupling in this core hole excitation leads to predominantly inelastic scattering and localization of the excited vibrations on the molecule on a femtosecond time scale. The coupling extends throughout the widths of the frontier valence bands.
Please use this url to cite or link to this publication:
https://lup.lub.lu.se/record/631059
- author
- Kjeldgaard, Lisbeth
LU
; Käämbre, Tanel
LU
; Schiessling, Joachim
; Marenne, Ingrid
; O'Shea, James N.
; Schnadt, Joachim
LU
; Glover, Chris J.
; Nagasono, Mitsuru
; Nordlund, Dennis
and Garnier, M. Gunnar
, et al. (More)
- Kjeldgaard, Lisbeth
LU
; Käämbre, Tanel
LU
; Schiessling, Joachim
; Marenne, Ingrid
; O'Shea, James N.
; Schnadt, Joachim
LU
; Glover, Chris J.
; Nagasono, Mitsuru
; Nordlund, Dennis
; Garnier, M. Gunnar
; Qian, Limin
; Rubensson, Jan-Erik
; Rudolf, Petra
; Mårtensson, Nils
LU
; Nordgren, Joseph
and Brühwiler, Paul A.
(Less)
- organization
- publishing date
- 2005
- type
- Contribution to journal
- publication status
- published
- subject
- in
- Physical Review B (Condensed Matter and Materials Physics)
- volume
- 72
- issue
- 20
- article number
- 205414
- publisher
- American Physical Society
- external identifiers
-
- wos:000233603900108
- scopus:29744447449
- ISSN
- 1098-0121
- DOI
- 10.1103/PhysRevB.72.205414
- language
- English
- LU publication?
- yes
- id
- df637402-7726-44e8-addb-175c45a43c7b (old id 631059)
- date added to LUP
- 2016-04-01 15:27:34
- date last changed
- 2025-04-04 14:18:31
@article{df637402-7726-44e8-addb-175c45a43c7b,
abstract = {{Vibronic coupling in solid C60 has been investigated with a combination of resonant photoemission spectroscopy (RPES) and resonant inelastic x-ray scattering (RIXS). Excitation as a function of energy within the lowest unoccupied molecular orbital resonance yielded strong oscillations in intensity and dispersion in RPES, and a strong inelastic component in RIXS. Reconciling these two observations establishes that vibronic coupling in this core hole excitation leads to predominantly inelastic scattering and localization of the excited vibrations on the molecule on a femtosecond time scale. The coupling extends throughout the widths of the frontier valence bands.}},
author = {{Kjeldgaard, Lisbeth and Käämbre, Tanel and Schiessling, Joachim and Marenne, Ingrid and O'Shea, James N. and Schnadt, Joachim and Glover, Chris J. and Nagasono, Mitsuru and Nordlund, Dennis and Garnier, M. Gunnar and Qian, Limin and Rubensson, Jan-Erik and Rudolf, Petra and Mårtensson, Nils and Nordgren, Joseph and Brühwiler, Paul A.}},
issn = {{1098-0121}},
language = {{eng}},
number = {{20}},
publisher = {{American Physical Society}},
series = {{Physical Review B (Condensed Matter and Materials Physics)}},
title = {{Intramolecular vibronic dynamics in molecular solids: C60}},
url = {{http://dx.doi.org/10.1103/PhysRevB.72.205414}},
doi = {{10.1103/PhysRevB.72.205414}},
volume = {{72}},
year = {{2005}},
}