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Continuous rotary membrane emulsification for the production of sustainable Pickering emulsions

Ekanem, Ekanem E. ; Wilson, Amy ; Scott, Janet L. ; Edler, Karen J. LU orcid and Mattia, Davide (2022) In Chemical Engineering Science 249.
Abstract

A continuous rotary membrane emulsification (cRME) system, allowing the decoupling of droplet generation from continuous phase (CP) flowrate, is presented here for the first time. The decoupling results in higher productivity and greater control compared to traditional crossflow and rotational membrane emulsification processes. A design of experiment (DoE) investigated the influence on droplet formation of CP flow, membrane rotational speed and emulsion composition, using a Pickering emulsion consisting of 1 wt% keratin solution and varying concentrations of oxidised cellulose nanofibrils. Experiments showed that CP flowrate had a negligible effect on droplet diameters in a wide range (between 78 and 241 µm), with uniformity index as... (More)

A continuous rotary membrane emulsification (cRME) system, allowing the decoupling of droplet generation from continuous phase (CP) flowrate, is presented here for the first time. The decoupling results in higher productivity and greater control compared to traditional crossflow and rotational membrane emulsification processes. A design of experiment (DoE) investigated the influence on droplet formation of CP flow, membrane rotational speed and emulsion composition, using a Pickering emulsion consisting of 1 wt% keratin solution and varying concentrations of oxidised cellulose nanofibrils. Experiments showed that CP flowrate had a negligible effect on droplet diameters in a wide range (between 78 and 241 µm), with uniformity index as low as 0.14 for optimal membrane rotational speeds and different oxidised cellulose nanofibrils (OCNF) concentration.

cRME has the potential to overcome low emulsion concentration limitations of continuous membrane emulsification systems, paving the way to significantly increase the productivity and application in personal care, food and drugs industries.

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author
; ; ; and
publishing date
type
Contribution to journal
publication status
published
subject
keywords
3-D printing, Monodisperse emulsion, Pickering emulsions, Rotary membrane emulsification, Stainless steel membrane, Sustainability
in
Chemical Engineering Science
volume
249
article number
117328
pages
11 pages
publisher
Elsevier
external identifiers
  • scopus:85121236111
ISSN
0009-2509
DOI
10.1016/j.ces.2021.117328
language
English
LU publication?
no
additional info
Publisher Copyright: © 2021 Elsevier Ltd
id
6963b785-a22b-4c61-9bca-d25488b176d5
date added to LUP
2022-07-12 15:32:38
date last changed
2022-07-29 12:56:40
@article{6963b785-a22b-4c61-9bca-d25488b176d5,
  abstract     = {{<p>A continuous rotary membrane emulsification (cRME) system, allowing the decoupling of droplet generation from continuous phase (CP) flowrate, is presented here for the first time. The decoupling results in higher productivity and greater control compared to traditional crossflow and rotational membrane emulsification processes. A design of experiment (DoE) investigated the influence on droplet formation of CP flow, membrane rotational speed and emulsion composition, using a Pickering emulsion consisting of 1 wt% keratin solution and varying concentrations of oxidised cellulose nanofibrils. Experiments showed that CP flowrate had a negligible effect on droplet diameters in a wide range (between 78 and 241 µm), with uniformity index as low as 0.14 for optimal membrane rotational speeds and different oxidised cellulose nanofibrils (OCNF) concentration. <br/></p><p>cRME has the potential to overcome low emulsion concentration limitations of continuous membrane emulsification systems, paving the way to significantly increase the productivity and application in personal care, food and drugs industries.</p>}},
  author       = {{Ekanem, Ekanem E. and Wilson, Amy and Scott, Janet L. and Edler, Karen J. and Mattia, Davide}},
  issn         = {{0009-2509}},
  keywords     = {{3-D printing; Monodisperse emulsion; Pickering emulsions; Rotary membrane emulsification; Stainless steel membrane; Sustainability}},
  language     = {{eng}},
  month        = {{02}},
  publisher    = {{Elsevier}},
  series       = {{Chemical Engineering Science}},
  title        = {{Continuous rotary membrane emulsification for the production of sustainable Pickering emulsions}},
  url          = {{http://dx.doi.org/10.1016/j.ces.2021.117328}},
  doi          = {{10.1016/j.ces.2021.117328}},
  volume       = {{249}},
  year         = {{2022}},
}