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Flame structure and burning velocity of ammonia/air turbulent premixed flames at high Karlovitz number conditions

Fan, Qingshuang LU ; Liu, Xin LU ; Xu, Leilei LU ; Subash, Arman Ahamed LU ; Brackmann, Christian LU ; Aldén, Marcus LU ; Bai, Xue Song LU and Li, Zhongshan LU (2022) In Combustion and Flame 238.
Abstract

This paper presents experimental studies of the structures and burning velocities of premixed ammonia/air jet flames at high Karlovitz (Ka) number conditions. Simultaneous planar laser-induced fluorescence (PLIF) imaging of imidogen (NH) and hydroxyl (OH) radicals was performed to investigate the local flame structure and Laser Doppler Anemometry (LDA) measurements were employed for extracting complement relevant turbulent quantities from the flow field. All the selected cases are located in the regime of distributed reaction zones (DRZ) in the Borghi-Peters diagram, with a maximum Karlovitz (Ka) number and turbulent intensity (u/SL) up to 1008 and 240, respectively. The OH- and NH-PLIF data were used to determine... (More)

This paper presents experimental studies of the structures and burning velocities of premixed ammonia/air jet flames at high Karlovitz (Ka) number conditions. Simultaneous planar laser-induced fluorescence (PLIF) imaging of imidogen (NH) and hydroxyl (OH) radicals was performed to investigate the local flame structure and Laser Doppler Anemometry (LDA) measurements were employed for extracting complement relevant turbulent quantities from the flow field. All the selected cases are located in the regime of distributed reaction zones (DRZ) in the Borghi-Peters diagram, with a maximum Karlovitz (Ka) number and turbulent intensity (u/SL) up to 1008 and 240, respectively. The OH- and NH-PLIF data were used to determine the flame surface density, flame-surface area ratio, and turbulent burning velocity (ST). The main findings include: (a) The NH layer remains thin and continuous over the investigated range of turbulent intensity and Karlovitz number, and the thickness keeps constant statistically without any significant broadening by turbulent eddies; (b) Spatial correlations of the NH and OH radicals show that overlap of NH and OH layers always exists in a thin region where OH has a weaker signal intensity; (c) The ratio of turbulent to laminar burning velocity (ST/SL) shows a nearly linear increase with turbulent intensity, while the ratio of wrinkled flame surface area to that of ensemble-averaged flame surface area increases only slightly with turbulent intensities. The slower increase of wrinkled flame surface area with turbulent intensity can be attributed to under-resolution in the current state-of-the-art PLIF experiments, the neglection of 3D flame wrinkles in 2D experiments, and the increase in flame stretch factor at high turbulent intensities.

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author
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organization
publishing date
type
Contribution to journal
publication status
published
subject
keywords
Flame structures, High Karlovitz Ka, Laser diagnostics, Premixed ammonia/air flames, Turbulent burning velocity
in
Combustion and Flame
volume
238
article number
111943
publisher
Elsevier
external identifiers
  • scopus:85122081734
ISSN
0010-2180
DOI
10.1016/j.combustflame.2021.111943
language
English
LU publication?
yes
additional info
Publisher Copyright: © 2021 The Authors
id
7e3c27dd-85f1-47be-9c2a-c4c581000073
date added to LUP
2022-01-26 09:27:13
date last changed
2024-03-09 03:05:29
@article{7e3c27dd-85f1-47be-9c2a-c4c581000073,
  abstract     = {{<p>This paper presents experimental studies of the structures and burning velocities of premixed ammonia/air jet flames at high Karlovitz (Ka) number conditions. Simultaneous planar laser-induced fluorescence (PLIF) imaging of imidogen (NH) and hydroxyl (OH) radicals was performed to investigate the local flame structure and Laser Doppler Anemometry (LDA) measurements were employed for extracting complement relevant turbulent quantities from the flow field. All the selected cases are located in the regime of distributed reaction zones (DRZ) in the Borghi-Peters diagram, with a maximum Karlovitz (Ka) number and turbulent intensity (u<sup>′</sup>/S<sub>L</sub>) up to 1008 and 240, respectively. The OH- and NH-PLIF data were used to determine the flame surface density, flame-surface area ratio, and turbulent burning velocity (S<sub>T</sub>). The main findings include: (a) The NH layer remains thin and continuous over the investigated range of turbulent intensity and Karlovitz number, and the thickness keeps constant statistically without any significant broadening by turbulent eddies; (b) Spatial correlations of the NH and OH radicals show that overlap of NH and OH layers always exists in a thin region where OH has a weaker signal intensity; (c) The ratio of turbulent to laminar burning velocity (S<sub>T</sub>/S<sub>L</sub>) shows a nearly linear increase with turbulent intensity, while the ratio of wrinkled flame surface area to that of ensemble-averaged flame surface area increases only slightly with turbulent intensities. The slower increase of wrinkled flame surface area with turbulent intensity can be attributed to under-resolution in the current state-of-the-art PLIF experiments, the neglection of 3D flame wrinkles in 2D experiments, and the increase in flame stretch factor at high turbulent intensities.</p>}},
  author       = {{Fan, Qingshuang and Liu, Xin and Xu, Leilei and Subash, Arman Ahamed and Brackmann, Christian and Aldén, Marcus and Bai, Xue Song and Li, Zhongshan}},
  issn         = {{0010-2180}},
  keywords     = {{Flame structures; High Karlovitz Ka; Laser diagnostics; Premixed ammonia/air flames; Turbulent burning velocity}},
  language     = {{eng}},
  publisher    = {{Elsevier}},
  series       = {{Combustion and Flame}},
  title        = {{Flame structure and burning velocity of ammonia/air turbulent premixed flames at high Karlovitz number conditions}},
  url          = {{http://dx.doi.org/10.1016/j.combustflame.2021.111943}},
  doi          = {{10.1016/j.combustflame.2021.111943}},
  volume       = {{238}},
  year         = {{2022}},
}