A physics-based micromechanical model for electroactive viscoelastic polymers
(2018) In Journal of Intelligent Material Systems and Structures 29(14). p.2902-2918- Abstract
Electroactive polymers with time-dependent behavior are considered in the present paper by way of a new physics-based micromechanical model; such viscoelastic response is described by the internal evolution of the polymer network, providing a new viewpoint on the stress relaxation occurring in elastomers. The main peculiarity of such internally rearranging materials is their capacity to locally reset their reference stress-free state, leading to a mechanical behavior that relaxes out (eases off) an induced stress state and that can thus be assimilated to a sort of internal self-healing process. Such high deformability and recoverability displayed by dynamically cross-linked polymers can be conveniently exploited when they are coupled in... (More)
Electroactive polymers with time-dependent behavior are considered in the present paper by way of a new physics-based micromechanical model; such viscoelastic response is described by the internal evolution of the polymer network, providing a new viewpoint on the stress relaxation occurring in elastomers. The main peculiarity of such internally rearranging materials is their capacity to locally reset their reference stress-free state, leading to a mechanical behavior that relaxes out (eases off) an induced stress state and that can thus be assimilated to a sort of internal self-healing process. Such high deformability and recoverability displayed by dynamically cross-linked polymers can be conveniently exploited when they are coupled in electromechanical problems; the deformation induced by an electric field can be easily tuned by the intensity of the electric field itself and the obtained shape can be maintained without any electric influence once the material microstructure has rearranged after a sufficient curing time. In the present paper, both features of the polymeric material, that is, internal remodeling and electromechanical coupled response, are considered and a theoretical framework is established to simulate representative boundary value problems.
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- author
- Brighenti, Roberto ; Menzel, Andreas LU and Vernerey, Franck J.
- organization
- publishing date
- 2018-08
- type
- Contribution to journal
- publication status
- published
- subject
- keywords
- cross-link evolution, Electroactive polymers, electromechanical coupling, morphing
- in
- Journal of Intelligent Material Systems and Structures
- volume
- 29
- issue
- 14
- pages
- 2902 - 2918
- publisher
- SAGE Publications
- external identifiers
-
- scopus:85049900675
- ISSN
- 1045-389X
- DOI
- 10.1177/1045389X18781036
- language
- English
- LU publication?
- yes
- id
- 7f889959-22c1-4ee6-a86a-a990c8823443
- date added to LUP
- 2018-08-02 09:31:49
- date last changed
- 2022-04-02 01:26:08
@article{7f889959-22c1-4ee6-a86a-a990c8823443,
abstract = {{<p>Electroactive polymers with time-dependent behavior are considered in the present paper by way of a new physics-based micromechanical model; such viscoelastic response is described by the internal evolution of the polymer network, providing a new viewpoint on the stress relaxation occurring in elastomers. The main peculiarity of such internally rearranging materials is their capacity to locally reset their reference stress-free state, leading to a mechanical behavior that relaxes out (eases off) an induced stress state and that can thus be assimilated to a sort of internal self-healing process. Such high deformability and recoverability displayed by dynamically cross-linked polymers can be conveniently exploited when they are coupled in electromechanical problems; the deformation induced by an electric field can be easily tuned by the intensity of the electric field itself and the obtained shape can be maintained without any electric influence once the material microstructure has rearranged after a sufficient curing time. In the present paper, both features of the polymeric material, that is, internal remodeling and electromechanical coupled response, are considered and a theoretical framework is established to simulate representative boundary value problems.</p>}},
author = {{Brighenti, Roberto and Menzel, Andreas and Vernerey, Franck J.}},
issn = {{1045-389X}},
keywords = {{cross-link evolution; Electroactive polymers; electromechanical coupling; morphing}},
language = {{eng}},
number = {{14}},
pages = {{2902--2918}},
publisher = {{SAGE Publications}},
series = {{Journal of Intelligent Material Systems and Structures}},
title = {{A physics-based micromechanical model for electroactive viscoelastic polymers}},
url = {{http://dx.doi.org/10.1177/1045389X18781036}},
doi = {{10.1177/1045389X18781036}},
volume = {{29}},
year = {{2018}},
}