Development of Perovskite Nanocrystal Superlattices for Studies of Collective Phenomena
Tallarini, Lorenzo LU ; Gomes Ferreira, Matheus LU
and Baranov, Dmitry
LU
(2024)
MATSUS24: The Materials for Sustainable Development Conference
- Abstract
- Colloidal perovskite nanocrystals are building blocks for novel materials due to the property of nanocrystals to self-assemble into ordered structures (superlattices). Exemplified by a prototypical perovskite CsPbBr3, research into perovskite nanocrystal superlattices is motivated by reports of intriguing phenomena such as superfluorescence and superradiance.[1] Such cooperative luminescence arises from the radiative coupling due to the interactions between individual nanocrystals (e.g., dipole-dipole) and between nanocrystals and the common electromagnetic field.
Different collective behaviors are expected from superlattices made from nanocrystals of different sizes because of quantum confinement effects. In recent theoretical... (More) - Colloidal perovskite nanocrystals are building blocks for novel materials due to the property of nanocrystals to self-assemble into ordered structures (superlattices). Exemplified by a prototypical perovskite CsPbBr3, research into perovskite nanocrystal superlattices is motivated by reports of intriguing phenomena such as superfluorescence and superradiance.[1] Such cooperative luminescence arises from the radiative coupling due to the interactions between individual nanocrystals (e.g., dipole-dipole) and between nanocrystals and the common electromagnetic field.
Different collective behaviors are expected from superlattices made from nanocrystals of different sizes because of quantum confinement effects. In recent theoretical work, the role of nanocrystal parameters such as nanocrystal size, size distribution, and interparticle distances onto single-excitation superradiance have been explored.[2] The first step in testing the theoretical predictions is to produce and characterize superlattices with desired structural parameters. In this work, we will discuss preparing and characterizing CsPbBr3 nanocrystal superlattices made from strongly and moderately confined nanocrystals (ca. 5-6 nm and 10-11 nm, respectively), and address their prospects as platforms for experimental tests of the predicted superradiance.
(Less)
Please use this url to cite or link to this publication:
https://lup.lub.lu.se/record/a8bea5b1-61a2-4cea-88a6-83abf2088aaf
- author
- Tallarini, Lorenzo
LU
; Gomes Ferreira, Matheus
LU
and Baranov, Dmitry
LU
- organization
- publishing date
- 2024-03-04
- type
- Contribution to conference
- publication status
- unpublished
- conference name
- MATSUS24: The Materials for Sustainable Development Conference
- conference location
- Barcelona, Spain
- conference dates
- 2024-03-04 - 2024-03-08
- project
- Engineering of Superfluorescent Nanocrystal Solids
- language
- English
- LU publication?
- yes
- id
- a8bea5b1-61a2-4cea-88a6-83abf2088aaf
- date added to LUP
- 2024-03-18 10:02:17
- date last changed
- 2024-03-22 13:57:17
@misc{a8bea5b1-61a2-4cea-88a6-83abf2088aaf,
abstract = {{Colloidal perovskite nanocrystals are building blocks for novel materials due to the property of nanocrystals to self-assemble into ordered structures (superlattices). Exemplified by a prototypical perovskite CsPbBr3, research into perovskite nanocrystal superlattices is motivated by reports of intriguing phenomena such as superfluorescence and superradiance.[1] Such cooperative luminescence arises from the radiative coupling due to the interactions between individual nanocrystals (e.g., dipole-dipole) and between nanocrystals and the common electromagnetic field.<br/><br/>Different collective behaviors are expected from superlattices made from nanocrystals of different sizes because of quantum confinement effects. In recent theoretical work, the role of nanocrystal parameters such as nanocrystal size, size distribution, and interparticle distances onto single-excitation superradiance have been explored.[2] The first step in testing the theoretical predictions is to produce and characterize superlattices with desired structural parameters. In this work, we will discuss preparing and characterizing CsPbBr3 nanocrystal superlattices made from strongly and moderately confined nanocrystals (ca. 5-6 nm and 10-11 nm, respectively), and address their prospects as platforms for experimental tests of the predicted superradiance.<br/>}},
author = {{Tallarini, Lorenzo and Gomes Ferreira, Matheus and Baranov, Dmitry}},
language = {{eng}},
month = {{03}},
title = {{Development of Perovskite Nanocrystal Superlattices for Studies of Collective Phenomena}},
year = {{2024}},
}