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Spatial quantum beats in vibrational resonant inelastic soft x-ray scattering at dissociating States in oxygen.

Pietzsch, Annette LU ; Sun, Y ; Hennies, Franz LU ; Rinkevicius, Z ; Karlsson, H O ; Schmitt, T ; Strocov, V N ; Andersson, J ; Kennedy, B and Schlappa, J , et al. (2011) In Physical Review Letters 106(15).
Abstract
Resonant inelastic soft x-ray scattering (RIXS) spectra excited at the 1σ_{g}→3σ_{u} resonance in gas-phase O_{2} show excitations due to the nuclear degrees of freedom with up to 35 well-resolved discrete vibronic states and a continuum due to the kinetic energy distribution of the separated atoms. The RIXS profile demonstrates spatial quantum beats caused by two interfering wave packets with different momenta as the atoms separate. Thomson scattering strongly affects both the spectral profile and the scattering anisotropy.
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author
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organization
publishing date
type
Contribution to journal
publication status
published
subject
in
Physical Review Letters
volume
106
issue
15
article number
153004
publisher
American Physical Society
external identifiers
  • wos:000289525300005
  • pmid:21568552
  • scopus:79960623604
  • pmid:21568552
ISSN
1079-7114
DOI
10.1103/PhysRevLett.106.153004
language
English
LU publication?
yes
id
c20646eb-7b68-4122-9cc2-6a41c76f35a5 (old id 1972639)
date added to LUP
2016-04-01 10:36:19
date last changed
2022-04-04 19:37:29
@article{c20646eb-7b68-4122-9cc2-6a41c76f35a5,
  abstract     = {{Resonant inelastic soft x-ray scattering (RIXS) spectra excited at the 1σ_{g}→3σ_{u} resonance in gas-phase O_{2} show excitations due to the nuclear degrees of freedom with up to 35 well-resolved discrete vibronic states and a continuum due to the kinetic energy distribution of the separated atoms. The RIXS profile demonstrates spatial quantum beats caused by two interfering wave packets with different momenta as the atoms separate. Thomson scattering strongly affects both the spectral profile and the scattering anisotropy.}},
  author       = {{Pietzsch, Annette and Sun, Y and Hennies, Franz and Rinkevicius, Z and Karlsson, H O and Schmitt, T and Strocov, V N and Andersson, J and Kennedy, B and Schlappa, J and Föhlisch, A and Rubensson, J-E and Gel'mukhanov, F}},
  issn         = {{1079-7114}},
  language     = {{eng}},
  number       = {{15}},
  publisher    = {{American Physical Society}},
  series       = {{Physical Review Letters}},
  title        = {{Spatial quantum beats in vibrational resonant inelastic soft x-ray scattering at dissociating States in oxygen.}},
  url          = {{http://dx.doi.org/10.1103/PhysRevLett.106.153004}},
  doi          = {{10.1103/PhysRevLett.106.153004}},
  volume       = {{106}},
  year         = {{2011}},
}