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A spatiotemporal ensemble model to predict gross beta particulate radioactivity across the contiguous United States

Li, Longxiang ; Blomberg, Annelise J. LU orcid ; Lawrence, Joy ; Réquia, Weeberb J. ; Wei, Yaguang ; Liu, Man ; Peralta, Adjani A. and Koutrakis, Petros (2021) In Environment International 156.
Abstract

Particulate radioactivity, a characteristic of particulate matter, is primarily determined by the abundance of radionuclides that are bound to airborne particulates. Exposure to high levels of particulate radioactivity has been associated with negative health outcomes. However, there are currently no spatially and temporally resolved particulate radioactivity data for exposure assessment purposes. We estimated the monthly distributions of gross beta particulate radioactivity across the contiguous United States from 2001 to 2017 with a spatial resolution of 32 km, via a multi-stage ensemble-based model. Particulate radioactivity was measured at 129 RadNet monitors across the contiguous U.S. In stage one, we built 264 base learning models... (More)

Particulate radioactivity, a characteristic of particulate matter, is primarily determined by the abundance of radionuclides that are bound to airborne particulates. Exposure to high levels of particulate radioactivity has been associated with negative health outcomes. However, there are currently no spatially and temporally resolved particulate radioactivity data for exposure assessment purposes. We estimated the monthly distributions of gross beta particulate radioactivity across the contiguous United States from 2001 to 2017 with a spatial resolution of 32 km, via a multi-stage ensemble-based model. Particulate radioactivity was measured at 129 RadNet monitors across the contiguous U.S. In stage one, we built 264 base learning models using six methods, then selected nine base models that provide different predictions. In stage two, we used a non-negative geographically and temporally weighted regression method to aggregate the selected base learner predictions based on their local performance. The results of block cross-validation analysis suggested that the non-negative geographically and temporally weighted regression ensemble learning model outperformed all base learning model with the smallest rooted mean square error (0.094 mBq/m3). Our model provided an accurate estimation of particulate radioactivity, thus can be used in future health studies.

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author
; ; ; ; ; ; and
organization
publishing date
type
Contribution to journal
publication status
published
subject
keywords
Geographically and temporally weighted regression, Particulate radioactivity, Spatiotemporal ensemble learning, Statistical learning
in
Environment International
volume
156
article number
106643
publisher
Elsevier
external identifiers
  • scopus:85110423911
  • pmid:34020300
ISSN
0160-4120
DOI
10.1016/j.envint.2021.106643
language
English
LU publication?
yes
id
f3688726-e6bb-4f32-9785-f65074ff5737
date added to LUP
2021-08-19 14:58:15
date last changed
2024-07-13 17:09:39
@article{f3688726-e6bb-4f32-9785-f65074ff5737,
  abstract     = {{<p>Particulate radioactivity, a characteristic of particulate matter, is primarily determined by the abundance of radionuclides that are bound to airborne particulates. Exposure to high levels of particulate radioactivity has been associated with negative health outcomes. However, there are currently no spatially and temporally resolved particulate radioactivity data for exposure assessment purposes. We estimated the monthly distributions of gross beta particulate radioactivity across the contiguous United States from 2001 to 2017 with a spatial resolution of 32 km, via a multi-stage ensemble-based model. Particulate radioactivity was measured at 129 RadNet monitors across the contiguous U.S. In stage one, we built 264 base learning models using six methods, then selected nine base models that provide different predictions. In stage two, we used a non-negative geographically and temporally weighted regression method to aggregate the selected base learner predictions based on their local performance. The results of block cross-validation analysis suggested that the non-negative geographically and temporally weighted regression ensemble learning model outperformed all base learning model with the smallest rooted mean square error (0.094 mBq/m<sup>3</sup>). Our model provided an accurate estimation of particulate radioactivity, thus can be used in future health studies.</p>}},
  author       = {{Li, Longxiang and Blomberg, Annelise J. and Lawrence, Joy and Réquia, Weeberb J. and Wei, Yaguang and Liu, Man and Peralta, Adjani A. and Koutrakis, Petros}},
  issn         = {{0160-4120}},
  keywords     = {{Geographically and temporally weighted regression; Particulate radioactivity; Spatiotemporal ensemble learning; Statistical learning}},
  language     = {{eng}},
  publisher    = {{Elsevier}},
  series       = {{Environment International}},
  title        = {{A spatiotemporal ensemble model to predict gross beta particulate radioactivity across the contiguous United States}},
  url          = {{http://dx.doi.org/10.1016/j.envint.2021.106643}},
  doi          = {{10.1016/j.envint.2021.106643}},
  volume       = {{156}},
  year         = {{2021}},
}